Contribution of black carbon to nonlinearity of sorption and desorption of acetochlor on sediment

doi:10.1007/s11783-008-0076-y

Front Envir Sci Eng Chin

2009, Vol. 3

Issue (1) : 69-74 https://doi.org/10.1007/s11783-008-0076-y

Research Article

Contribution of black carbon to nonlinearity of sorption and desorption of acetochlor on sediment

Jianqiu LIU, Yaobin ZHANG(

), Hong CHEN, Yazhi ZHAO, Xie QUAN

Key Laboratory of Industrial Ecology and Environmental Engineering

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Abstract

In order to investigate the contribution of various black carbon (BC) contents to nonlinearity of sorption and desorption isotherms for acetochlor on sediment, equilibrium sorption and desorption isotherms were determined to measure sorption and desorption of acetochlor in sediment amended with various amounts of BC. In this paper, two types of BC referred to as BC400 and BC500 were prepared at 400°C and 500°C, respectively. Higher preparation temperature facilitated the formation of micropores on BC to enhance its sorption capacity. Increase of the BC content obviously increased the sorption amount and reduced the desorption amount for acetochlor. When the BC500 contents in total organic carbon (TOC) increased from 0 to 60%, Freundlich sorption coefficient (K_f) increased from 4.07 to 35.74, and desorption hysteresis became gradually obvious. When the content of BC in TOC was lower than 23%, the sorption isotherm had a significant linear correlation (p = 0.05). In case of desorption, a significant nonlinear change could be observed when the content of BC was up to 13%. Increase of BC content in the sediment would result in shifting the sorption-desorption isotherms from linearity to nonlinearity, which indicated that contribution of BC to nonlinear adsorption fraction became gradually remarkable.

Keywords black carbon (BC) sorption desorption sediment

Corresponding Author(s): ZHANG Yaobin,Email:zhangyb@dlut.edu.cn

Issue Date: 05 March 2009

Cite this article:

Jianqiu LIU,Yaobin ZHANG,Hong CHEN, et al. Contribution of black carbon to nonlinearity of sorption and desorption of acetochlor on sediment[J]. Front Envir Sci Eng Chin, 2009, 3(1): 69-74.

URL:

https://academic.hep.com.cn/fese/EN/10.1007/s11783-008-0076-y
https://academic.hep.com.cn/fese/EN/Y2009/V3/I1/69

Tab0 Characteristics of two types of BC

Fig0 Freundlich sorption isotherms on the sediment amended with BC400 and BC500

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