Nanosized magnetite in low cost materials for remediation of water polluted with toxic metals, azo- and antraquinonic dyes

doi:10.1007/s11783-015-0814-x

Front. Environ. Sci. Eng.

2015, Vol. 9

Issue (5) : 746-769 https://doi.org/10.1007/s11783-015-0814-x

REVIEW ARTICLE

Nanosized magnetite in low cost materials for remediation of water polluted with toxic metals, azo- and antraquinonic dyes

María Fernanda HORST^1,^*(

),Verónica LASSALLE¹,María Luján FERREIRA²

1. Institute of Chemistry of the South (Inquisur, Universidad Nacional del Sur—CONICET), Avda Alem 1253, Bahía Blanca, Argentina
2. Pilot Plant of Chemical Engineering (PLAPIQUI-UNS-CONICET), Universidad Nacional del Sur—CONICET, Camino La Carrindanga km7, Bahía Blanca, Argentina

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Abstract

Nanosized magnetite has emerged as an adsorbent of pollutants in water remediation. Nanoadsorbents include magnetic iron oxide and its modifiers/stabilizers, such as carbon, silica, clay, organic moieties (polymers, aminoacids, and fatty acids) and other inorganic oxides. This review is focused on the recent developments on the synthesis and use of magnetic nanoparticles and nanocomposites in the treatment of contaminated water. The emphasis is on the influence of the iron oxide modifiers on some properties of interest such as size, BET area, and magnetization. The characteristics of these nanomaterials are related to their ability to eliminate heavy metal ions and dyes from wastewater. Comparative analysis of the actual literature was performed aiming to present the magnetic material, its preparation methodology and performance in the elimination of the selected pollutants. Vast information has been properly summarized according to the materials, their properties and preferential affinity for selected contaminants. The mechanisms governing nanomaterial’s formation as well as the interactions with heavy metals and dyes have been carefully analyzed and associated to their efficiency.

Keywords nanomagnetite water remediation toxic metals dyes supported magnetite

Corresponding Author(s): María Fernanda HORST

Online First Date: 14 September 2015 Issue Date: 08 October 2015

Cite this article:

María Luján FERREIRA,Verónica LASSALLE,María Fernanda HORST. Nanosized magnetite in low cost materials for remediation of water polluted with toxic metals, azo- and antraquinonic dyes[J]. Front. Environ. Sci. Eng., 2015, 9(5): 746-769.

URL:

https://academic.hep.com.cn/fese/EN/10.1007/s11783-015-0814-x
https://academic.hep.com.cn/fese/EN/Y2015/V9/I5/746

Tab.1 Different technologies applied to water remediation

Fig.1 Dyes analyzed in the manuscript. Sulfonic groups characterize anionic dyes whereas N=N, NH and NH₂ groups characterize cationic dyes

Fig.2 Local structure of magnetite

Fig.3 Scheme 1 Representation of co-precipitation method

Tab.2 Summarized characterization data of magnetite nanoparticles synthesized using different methods and its performance as heavy metals adsorbent

Fig.4 Mechanism of heavy metal ion adsorption onto magnetite nanoparticles

Fig.5 Evolution from peroxidase and catalase enzymes to nanozymes last 80 years

Fig.6 Schematic representation of elimination of heavy metals ions by ferrite method

Fig.7 Synthesis pathways of MNP with additives

Fig.8 The two mechanisms to surface modification of MNPs

Fig.9 Photographs of aqueous dispersions of MNPs modified with SDS in presence and absence of magnetic field

Fig.10 Interactions of heavy metals cations with magnetite nanoparticles and SDS

Fig.11 TEM micrograph of a CNT/Fe₃O₄

Fig.12 Representation of sol-gel or hydrothermal reaction synthesis for magnetic composites

Tab.3 Maximum adsorption of heavy metals using magnetic nanocomposites: graphene, carbon nanotubes, silica as a function of their properties

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