Recent progress in the interfacial polymerization process for CO<sub>2</sub> separation membrane fabrication

doi:10.1007/s11705-024-2510-5

Front. Chem. Sci. Eng.

2025, Vol. 19

Issue (1) : 3 https://doi.org/10.1007/s11705-024-2510-5

Recent progress in the interfacial polymerization process for CO₂ separation membrane fabrication

Zhijie Shang¹, Qiangqiang Song¹, Bin Han², Jing Ma¹, Dongyang Li¹, Cancan Zhang³, Xin Li⁴, Jinghe Yang¹, Junyong Zhu¹, Wenpeng Li¹(

), Jing Wang^1,⁵(

), Yatao Zhang^1,⁵

¹. School of Chemical Engineering, Zhengzhou University, Zhengzhou 450001, China
². Department of Radiation Oncology, The First Affiliated Hospital of Zhengzhou University, Zhengzhou 450052, China
³. MOE Key Laboratory of Enhanced Heat Transfer and Energy Conservation, Beijing Key Laboratory of Heat Transfer and Energy Conversion, Beijing University of Technology, Beijing 100124, China
⁴. Singapore Membrane Technology Centre, Nanyang Environment and Water Research Institute, Nanyang Technological University, 1 Cleantech Loop, 637141, Singapore
⁵. State Key Laboratory of Coking Coal Resources Green Exploitation, Zhengzhou University, Zhengzhou 450001, China

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Abstract

Nowadays, global warming caused by the increasing levels of CO₂ has become a serious environmental problem. Membrane separation technology has demonstrated its promising potential in carbon capture due to its easy operation, energy-efficientness and high efficiency. Interfacial polymerization process, as a facile and well-established technique for preparing membranes with a thin selective layer, has been widely used for fabricating commercial reverse osmosis and nanofiltration membranes in water treatment domain. To push forward such an interfacial polymerization process in the research of CO₂ separation membranes, herein we make a review on the regulation and research progress of the interfacial polymerization membranes for CO₂ separation. First, a comprehensive and critical review of the progress in the monomers, nanoparticles and interfacial polymerization process optimization for preparing CO₂ separation membrane is presented. In addition, the potential of molecular dynamics simulation and machine learning in accelerating the screen and design of interfacial polymerization membranes for CO₂ separation are outlined. Finally, the possible challenges and development prospects of CO₂ separation membranes by interfacial polymerization process are proposed. It is believed that this review can offer valuable insights and guidance for the future advancement of interfacial polymerization membranes for CO₂ separation, thereby fostering its development.

Keywords interfacial polymerization CO₂ separation monomer nanoparticle

Corresponding Author(s): Wenpeng Li,Jing Wang

Just Accepted Date: 18 July 2024 Issue Date: 28 November 2024

Cite this article:

Zhijie Shang,Qiangqiang Song,Bin Han, et al. Recent progress in the interfacial polymerization process for CO₂ separation membrane fabrication[J]. Front. Chem. Sci. Eng., 2025, 19(1): 3.

URL:

https://academic.hep.com.cn/fcse/EN/10.1007/s11705-024-2510-5
https://academic.hep.com.cn/fcse/EN/Y2025/V19/I1/3

Fig.2 Synthesis of IP membrane and amine and hydroxyl group aqueous phase monomers.

Tab.1 Membranes synthesized by amine monomers and their performances^a)

Fig.3 (a) Synthesis of membrane from amine-end-capped PI oligomers and TMC and the three-dimensional (3D) view of an amorphous cell containing the cross-linked network; (b) schematic diagram of preparing the selective layer by the IP process. Reprinted with permission from Ref. [36], copyright 2021, American Chemical Society.

Tab.2 Membranes synthesized by hydroxyl monomers and their performance^a)

Fig.5 IP membranes synthesized by TMC with hydroxyl monomers. (a) TTSBI. Reprinted with permission from Ref. [47], copyright 2019, Elsevier. (b) CDs. Reprinted with permission from Ref. [54], copyright 2018, Wiley-Blackwell. (c) MEDβCD. Reprinted with permission from Ref. [51], copyright 2023, Elsevier.

Tab.3 Commonly used nanoparticles in IP membranes for CO₂ separation and their membrane performance^a)

Fig.8 Schematic of fabrication process of TFN membranes by embedding (a) PG. Reprinted with permission from Ref. [63], copyright 2017, Elsevier. (b) C-MWCNTs. Reprinted with permission from Ref. [60], copyright 2021, Elsevier. (c) UiO-66-NH₂. Reprinted with permission from Ref. [66], copyright 2021, American Chemical Society.

Fig.9 Schematic illustration of covalent bonds between PA and (a) NH₂-ZIF-8. Reprinted with permission from Ref. [69], copyright 2017, Elsevier. (b) TpPa-1. Reprinted with permission from Ref. [70], copyright 2022, Chemical Industry Press. (c) The process of forming IP membranes via the swelling-controlled nanofiller positioning method. Reprinted with permission from Ref. [68], copyright 2021, Elsevier. (d) The homogeneous distribution of GO/CNT within the PA layer, Reprinted with permission from Ref. [57], copyright 2019, Elsevier.

Fig.10 Process of preparing interlayer in IP process with (a) GQDs/N-GQDs. Reprinted with permission from Ref. [49], copyright 2022, Elsevier. (b) 2D MOF (Zn₂(bim)₄) nanosheets. Reprinted with permission from Ref. [90], copyright 2021, Elsevier.

Fig.11 Schematic diagram for the model design, development, and application. (a) Network structure of the multitask multilayer perception, (b) online learning process with the introduction of expert experience, (c) illustration of the model training and evaluation, and (d) interpretation of model and guided design of membranes. Reprinted with permission from Ref. [106], copyright 2022, American Chemical Society.

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