Microwave enhanced stabilization of copper in artificially contaminated soil

doi:10.1007/s11783-010-0290-2

Front Envir Sci Eng Chin

2011, Vol. 5

Issue (2) : 205-211 https://doi.org/10.1007/s11783-010-0290-2

RESEARCH ARTICLE

Microwave enhanced stabilization of copper in artificially contaminated soil

Hua ZHANG^1,2, Zhiliang ZHU¹(

), Noboru YOSHIKAWA²

1. State Key Laboratory of Pollution Control and Resource Reuse, Tongji University, Shanghai 200092, China; 2. Graduate School of Environmental Studies, Tohoku University, Sendai 980-8579, Japan

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Abstract

Microwave processing was used to stabilize copper ions in soil samples. Its effects on the stabilization efficiency were studied as a function of additive, microwave power, process time, and reaction atmosphere. The stabilization efficiency of the microwave process was evaluated based on the results of the toxicity characteristic leaching procedure (TCLP) test. The results showed that the optimal experimental condition contained a 700 W microwave power, 20 min process time and 3 iron wires as the additive, and that the highest stabilization efficiency level was more than 70%. In addition, the different reaction atmospheres showed no apparent effect on the stabilization efficiency of copper in the artificially contaminated soil. According to the result of the Tessier sequential extraction, the partial species of copper in the contaminated soil was deduced to transform from unstable species to stable states after the microwave process.

Keywords microwave copper stabilization

Corresponding Author(s): ZHU Zhiliang,Email:zzl@tongji.edu.cn

Issue Date: 05 June 2011

Cite this article:

Hua ZHANG,Zhiliang ZHU,Noboru YOSHIKAWA. Microwave enhanced stabilization of copper in artificially contaminated soil[J]. Front Envir Sci Eng Chin, 2011, 5(2): 205-211.

URL:

https://academic.hep.com.cn/fese/EN/10.1007/s11783-010-0290-2
https://academic.hep.com.cn/fese/EN/Y2011/V5/I2/205

Tab.1 ICP-MS instrumental parameters

Fig.1 stabilization of copper in soil at the different times (without microwave radiation)

Fig.2 Effect of iron wire on stabilization efficiency (microwave power: 700 W; reaction time: 20 min)

Fig.3 Effect of iron wire diameter on the stabilization efficiency of copper
(microwave power: 700 W; reaction time: 20 min)

Tab.2 Relationship of the different diameter (ID), numbers of iron wires (IN) and the highest temperatures during the microwave process (microwave power: 700w; reaction time: 20 min)

Fig.4 Effect of microwave power on the stabilization efficiency
(reaction time: 20 min; iron wire number: 3)

Fig.5 Function of reaction time and temperature in the different microwave power
(Reaction time: 20 min; iron wire number: 3)

Fig.6 Function of reaction time and stabilization efficiency
(microwave power: 700W; iron wire number: 3)

Fig.7 Speciation analysis of copper in contaminated soil before and after microwave process

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