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A simple unilateral homogenous PhOLEDs with enhanced efficiency and reduced efficiency roll-off |
Shaoqing ZHUANG, Wenzhi ZHANG, Xiao YANG, Lei WANG() |
Wuhan National Laboratory for Optoelectronics, School of Optical and Electronic Information, Huazhong University of Science and Technology, Wuhan 430074, China |
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Abstract In this paper, highly efficient phosphorescent organic lighting emitting diodes (PhOELDs) with low efficiency roll-off are demonstrated by using a unilateral homogenous device structure with wide band-gap material 4, 4', 4″-tri(N-carbazolyl)-triphenylamine (TCTA) as hole transporting layer and emitting layer (EML). The optimized blue device exhibits a high power efficiency of 40 lm/W, external quantum efficiency of 19.2% and current efficiency of 37.7 cd/A. More importantly, the device exhibits a low efficiency roll-off at 1000 cd/m2. In addition, the white homogenous PhOLEDs only exhibits the efficiency roll-off 5.6% and 17.5%, corresponding to the brightness of 1000 and 5000 cd/m2 respectively. These interesting results demonstrate that the simple unilateral homogenous device structure is a promising way to enhance the device efficiency and reduce the efficiency roll-off.
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Keywords
enhance efficiency
efficiency roll-off
unilateral homogenous structures
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Corresponding Author(s):
WANG Lei,Email:wanglei@mail.hust.edu.cn
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Issue Date: 05 December 2013
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1 |
Tang C W, VanSlyke S A. Organic electroluminescent diodes. Applied Physics Letters , 1987, 51(12): 913-915 doi: 10.1063/1.98799
|
2 |
Fukase A, Dao K L T, Kido J. High-efficiency organic electroluminescent devices using iridium complex emitter and arylamine-containing polymer buffer layer. Ploymers for Advanced Technologies , 2002, 13(8): 601-604 doi: 10.1002/pat.229
|
3 |
Tanaka D, Sasabe H, Li Y J, Su S J, Takeda T, Kido J. Ultra high efficiency green organic light-emitting devices. Japanese Journal of Applied Physics , 2007, 46(1): L10-L12 doi: 10.1143/JJAP.46.L10
|
4 |
Su S J, Tanaka D, Li Y J, Sasabe H, Takeda T, Kido J. Novel four-pyridylbenzene-armed biphenyls as electron-transport materials for phosphorescent OLEDs. Organic Letters , 2008, 10(5): 941-944 doi: 10.1021/ol7030872 pmid:18237184
|
5 |
Kim H, Cho N S, Oh H Y, Yang J H, Jeon W S, Park J S, Suh M C, Kwon J H. Highly efficient red phosphorescent dopants in organic light-emitting devices. Advanced Materials , 2011, 23(24): 2721-2726 doi: 10.1002/adma.201100405 pmid:21495090
|
6 |
Fan C H, Sun P, Su T H, Cheng C H. Host and dopant materials for idealized deep-red organic electrophosphorescence devices. Advanced Materials , 2011, 23(26): 2981-2985 doi: 10.1002/adma.201100610 pmid:21567483
|
7 |
Malliaras G G, Scott J C. The roles of injection and mobility in organic light emitting diodes. Journal of Applied Physics , 1998, 83(10): 5399-5403 doi: 10.1063/1.367369
|
8 |
Polikarpov E, Swensen J S, Chopra N, So F, Padmaperuma A B. An ambipolar phosphine oxide-based host for high power efficiency blue phosphorescent organic light emitting devices. Applied Physics Letters , 2009, 94(22): 223304 doi: 10.1063/1.3148642
|
9 |
Gong S, Chen Y, Luo J, Yang C, Zhong C, Qin J, Ma D. Bipolar tetraarylsilanes as universal hosts for blue, green, orange, and white electrophosphorescence with high efficiency and low efficiency roll-off. Advanced Functional Materials , 2011, 21(6): 1168-1178 doi: 10.1002/adfm.201002066
|
10 |
Chou H H, Cheng C H. A highly efficient universal bipolar host for blue, green, and red phosphorescent OLEDs. Advanced Materials , 2010, 22(22): 2468-2471 doi: 10.1002/adma.201000061 pmid:20446307
|
11 |
Xiao L, Su S J, Agata Y, Lan H, Kido J. Nearly 100% internal quantum efficiency in an organic blue-light electrophosphorescent device using a weak electron transporting material with a wide energy gap. Advanced Materials , 2009, 21(12): 1271-1274 doi: 10.1002/adma.200802034
|
12 |
Lee J H, Huang C L, Hsiao C H, Leung M K, Yang C C, Chao C C. Blue phosphorescent organic light-emitting device with double emitting layer. Applied Physics Letters , 2009, 94(22): 223301 doi: 10.1063/1.3147866
|
13 |
Zhang X W, Li J, Khan M, Zhang L, Jiang X Y, Haq K, Zhu W Q, Zhang Z L. Improved chromaticity and electron injection in a blue organic light-emitting device by using a dual electron-transport layer with hole-blocking function. Semiconductor Science and Technology , 2009, 24(7): 075021 doi: 10.1088/0268-1242/24/7/075021
|
14 |
Cai C, Su S J, Chiba T, Sasabe H, Pu Y J, Nakayama K, Kido J. Efficient low-driving-voltage blue phosphorescent homojunction organic light-emitting devices. Japanese Journal of Applied Physics , 2011, 50(4): 040204 doi: 10.1143/JJAP.50.040204
|
15 |
Tsuji H, Mitsui C, Sato Y, Nakamura E. Bis(carbazolyl)benzodifuran: a high-mobility ambipolar material for homojunction organic light-emitting diode devices. Advanced Materials , 2009, 21(37): 3776-3779 doi: 10.1002/adma.200900634
|
16 |
Wang Q, Tao Y, Qiao X, Chen J, Ma D, Yang C, Qin J. High-performance, phosphorescent, top-emitting organic light-emitting diodes with p-i-n homojunctions. Advanced Functional Materials , 2011, 21(9): 1681-1686 doi: 10.1002/adfm.201002229
|
17 |
Jang S E, Yook K S, Lee J Y. High power efficiency in simplified two layer blue phosphorescent organic light-emitting diodes. Organic Electronics , 2010, 11(6): 1154-1157 doi: 10.1016/j.orgel.2010.04.004
|
18 |
Qiao X, Tao Y, Wang Q, Ma D, Yang C, Wang L, Qin J, Wang F. Controlling charge balance and exciton recombination by bipolar host in single-layer organic light-emitting diodes. Journal of Applied Physics , 2010, 108(3): 034508 doi: 10.1063/1.3457672
|
19 |
Zhang H, Huo C, Zhang J, Zhang P, Tian W, Wang Y. Efficient single-layer electroluminescent device based on a bipolar emitting boron-containing material. Chemical Communications (Cambridge) , 2006, (3): 281-283 doi: 10.1039/b513918j
|
20 |
Seo J H, Lee S J, Seo B M, Moon S J, Lee K H, Park J K, Yoon S S, Kim Y K. White organic light-emitting diodes showing nearly 100% internal quantum efficiency. Organic Electronics , 2010, 11(11): 1759-1766 doi: 10.1016/j.orgel.2010.07.015
|
21 |
Chen H, Lee J, Shiau C. Electromagnetic modeling of organic light-emitting devices. Journal of Lightwave Technology , 2006, 24(6): 2450-2457 doi: 10.1109/JLT.2006.874591
|
22 |
Su S J, Chiba T, Takeda T, Kido J. Pyridine-containing triphenylbenzene derivatives with high electron mobility for highly efficient phosphorescent OLEDs. Advanced Materials , 2008, 20(11): 2125-2130 doi: 10.1002/adma.200701730
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