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Frontiers of Chemical Science and Engineering

ISSN 2095-0179

ISSN 2095-0187(Online)

CN 11-5981/TQ

Postal Subscription Code 80-969

2018 Impact Factor: 2.809

Front. Chem. Sci. Eng.    2009, Vol. 3 Issue (4) : 468-473    https://doi.org/10.1007/s11705-009-0257-7
Research articles
Experimental study on capturing CO 2 greenhouse gas by mixture of ammonia and soil
Ying WU,Yifei WANG,Qinghua ZENG,Xin GONG,Zunhong YU,
Key Laboratory of Coal Gasification of Ministry of Education, Institute of Clean Coal Technology, East China University of Science and Technology, Shanghai 200237, China;
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Abstract This paper presents our study on removal of carbon dioxide (CO2) greenhouse gas emissions by using the mixture of ammonia and soil. CO2 capture capacity using this method is 15% higher than the sum of ammonia chemical absorption capacity and soil physical adsorption capacity. Scanning electron microscopy (SEM) and Fourier transform infrared spectroscopy (FTIR) are utilized to study this synergism. The removal effect is not only reflected in ammonia chemical reaction with CO2. CO2 can also be absorbed by ammonium bicarbonate (NH4HCO3) crystal, which is the main component of the product, or wrapped in the pore of the crystal or packed in the gap between the crystal and the soil. CO2 can be permanently deposited as carbonated minerals in the subsoil earth layers.
Issue Date: 05 December 2009
 Cite this article:   
Yifei WANG,Ying WU,Qinghua ZENG, et al. Experimental study on capturing CO 2 greenhouse gas by mixture of ammonia and soil[J]. Front. Chem. Sci. Eng., 2009, 3(4): 468-473.
 URL:  
https://academic.hep.com.cn/fcse/EN/10.1007/s11705-009-0257-7
https://academic.hep.com.cn/fcse/EN/Y2009/V3/I4/468
Liu F, Wang S J, Chen C H, Xu X C. Researchprogress of CO2 capture by using ammonia fromflue gas of power plant. The Chemical Industryand Engineering Society of China, 2009, 60(2): 269–278 (in Chinese)
Diao Y F, Zheng X Y, He B S, Chen C H, Xu X C. Experimental study on capturing CO2 greenhouse gas by ammonia scrubbing. Energy Conversion and Management, 2004, 45: 2283–2296

doi: 10.1016/j.enconman.2003.10.011
Yeh A C, Bai H. Comparison of ammonia andmonoethanolamine solvents to reduce CO2 greenhousegas emissions. The Science of Total Environment, 1999, 228: 121–133

doi: 10.1016/S0048-9697(99)00025-X
Zhang M, Sai J C, Wu S H, Li Z Z. Experimentalstudy of the removal of CO2 from coal-firedflue gas by using ammonia. Journal of Engineeringfor the Thermal Energy and Power, 2008, 23(2): 191―194, 219 (in Chinese)
Dong J X, Zhang Y, Zhang Y, Jia Y G, Li Z Z, Li C F, Li Y L. Experimental study on absorptionof CO2 in flue gas by hydrous ammonia. Journal of Power Engineering, 2007, 27(3): 438–440 (in Chinese)
Zhang M, Chen H P, He Q, Zhang S H, Zheng C G. Experimental study on removal of carbondioxide from flue gas by aqueous ammonia. Energy and Environment, 2007, 4: 81–83 (in Chinese)
Bai H, Yeh A C. Removal of CO2 greenhouse gas by ammonia scrubbing. Industrial and Engineering Chemistry Research, 1997, 36: 2490–2493

doi: 10.1021/ie960748j
Zeng Q H, Wang Y F, Wu Y, Yu G S, Yu Z H. Study on removal of CO2 greenhouse gas by mixture of ammonia and soil. Journal of Environmental Engineering, 2009, 9: 1630–1634 (in Chinese)
Bao W J, Li H Q, Zhang Y. Progress in carbon dioxide sequestration by mineral carbonation. Journal of Chemical Industry and Engineering, 2007, 58(1): 1–9
Lee J W, Li R F. Integration of fossil energysystems with CO2 sequestration through NH4HCO3 production. Energy Conversion and Management, 2003, 44: 1535–1546

doi: 10.1016/S0196-8904(02)00149-8
Zhang Z M, Feng Y Q. New Nitrogenous Fertilizer:Long-Effect Ammonium Bicarbonate. Beijing: Chemical Industry Press, 2000 (in Chinese)
Yao S, Yang L J, Shen X L. New technique for CO2 mitigation:research of CO2 sequestration in soil. Journal of Southeast University (Natural ScienceEdition), 2004, 34(2): 228–231 (in Chinese)
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