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Frontiers of Chemical Science and Engineering

ISSN 2095-0179

ISSN 2095-0187(Online)

CN 11-5981/TQ

邮发代号 80-969

2019 Impact Factor: 3.552

Frontiers of Chemical Science and Engineering  2023, Vol. 17 Issue (6): 759-771   https://doi.org/10.1007/s11705-022-2269-5
  本期目录
Multiple input self-organizing-map ResNet model for optimization of petroleum refinery conversion units
Jiannan Zhu1, Vladimir Mahalec2, Chen Fan1, Minglei Yang1,3(), Feng Qian1,3()
1. Key Laboratory of Smart Manufacturing in Energy Chemical Process, Ministry of Education, East China University of Science and Technology, Shanghai 200237, China
2. Department of Chemical Engineering, McMaster University, Hamilton, Ontario L8S 4L8, Canada
3. Engineering Research Center of Process System Engineering, Ministry of Education, East China University of Science and Technology, Shanghai 200237, China
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Abstract

This work introduces a deep-learning network, i.e., multi-input self-organizing-map ResNet (MISR), for modeling refining units comprised of two reactors and a separation train. The model is comprised of self-organizing-map and the neural network parts. The self-organizing-map part maps the input data into multiple two-dimensional planes and sends them to the neural network part. In the neural network part, residual blocks enhance the convergence and accuracy, ensuring that the structure will not be overfitted easily. Development of the MISR model of hydrocracking unit also benefits from the utilization of prior knowledge of the importance of the input variables for predicting properties of the products. The results show that the proposed MISR structure predicts more accurately the product yields and properties than the previously introduced self-organizing-map convolutional neural network model, thus leading to more accurate optimization of the hydrocracker operation. Moreover, the MISR model has smoother error convergence than the previous model. Optimal operating conditions have been determined via multi-round-particle-swarm and differential evolution algorithms. Numerical experiments show that the MISR model is suitable for modeling nonlinear conversion units which are often encountered in refining and petrochemical plants.

Key wordshydrocracking    convolutional neural networks    self-organizing map    deep learning    data-driven optimization
收稿日期: 2022-06-29      出版日期: 2023-05-17
Corresponding Author(s): Minglei Yang,Feng Qian   
 引用本文:   
. [J]. Frontiers of Chemical Science and Engineering, 2023, 17(6): 759-771.
Jiannan Zhu, Vladimir Mahalec, Chen Fan, Minglei Yang, Feng Qian. Multiple input self-organizing-map ResNet model for optimization of petroleum refinery conversion units. Front. Chem. Sci. Eng., 2023, 17(6): 759-771.
 链接本文:  
https://academic.hep.com.cn/fcse/CN/10.1007/s11705-022-2269-5
https://academic.hep.com.cn/fcse/CN/Y2023/V17/I6/759
Fig.1  
CategoryDefinitionNumber
Inputs-feed 1 (VGO)True boiling points9
Density1
Sulfur content1
Nitrogen content1
Inputs-feed 2 (hydrotreated FCC diesel)True boiling points9
Density1
Sulfur content1
Nitrogen content1
Inputs-operating conditionsFeed ratio1
Hydrogen to oil ratio2
Reactor pressure1
Inlet temperatures8
OutputsYields8
Properties72
Tab.1  
Fig.2  
Index24 × 2432 × 3248 × 4896 × 96128 × 128
Executing time/min7.588.098.5117.3332.99
R2 (correlation coefficient)0.9500.9560.9530.96110.9606
Mean relative error (MRE)2.35871.96452.21861.81961.6652
Mean absolute error (MAE)0.42630.36100.37680.31710.2960
Tab.2  
Fig.3  
Fig.4  
IndexSOM-CNN without BNSOM-CNN with BN
Iterations20002000
Correlation coefficient R20.93290.9468
MRE (10 samples)2.5432.316
MAE (10 samples)0.49700.4464
Time cost/min5.507.66
Tab.3  
Fig.5  
IndexSOM-CNNMulti-input-SOM-CNN
Correlation coefficient R20.94680.9533
MRE (test samples)2.3162.117
MAE (test samples)0.44640.3870
Time cost/min7.668.01
Tab.4  
Fig.6  
Index2 residual blocks3 residual blocks4 residual blocks5 residual blocks
Loss0.001040.001020.001020.00100
Iterations2000200020002000
Total time/min19.725.933.170.8
Correlation coefficient R2 (total outputs)0.96280.96350.96380.9655
R2 (properties only)0.93690.93540.93680.9402
MRE (test samples)1.8621.69281.67101.6700
MAE (test samples)0.33710.31770.31950.3071
Number of trainable parameters378,4131,580,0006,379,00025,563,000
Tab.5  
Fig.7  
Index1 hidden layer2 hidden layers3 hidden layers4 hidden layers5 hidden layers
Structure36-64-1336-128-64-1336-128-128-64-1336-128-256-128-64-1336-128-256-256-128-64-13
Loss0.002110.001740.001610.001250.00120
Iterations50005000500050005000
Total time/min3.85.26.29.410.3
Correlation coefficient R2 (total outputs)0.9280.9390.9430.9540.956
R2 (properties only)0.8680.8900.8950.9150.917
MRE (test samples)2.6232.3282.2491.9991.914
MAE (test samples)0.5180.4700.4550.41870.4035
Number of trainable parameters3213138373034996269145549
Tab.6  
IndexFNNSOM-CNNMulti-input-SOM-CNNMISR with 3 residual blocks
Loss0.001610.001570.001270.00099
Iterations5000200020002000
Total time/min6.27.68.125.2
Correlation coefficient R2 (total outputs)0.94340.94180.95360.9638
R2 (properties only)0.8950.8920.9170.937
MRE2.2492.3321.9871.686
MAE0.4550.4560.3860.314
Tab.7  
Fig.8  
Fig.9  
Index1 round-PSO1 round-DEMulti-round-PSO
Rounds1140
Iterations per round4001000400
Total time/min2.06154.1682.54
Seconds per iteration0.319.250.31
Max profit (10 times)2420.392413.022429.67
Mean profit (10 times)2321.912395.192423.19
Tab.8  
Case numberSOM-CNN prediction benefitSOM-CNN real benefitSOM-CNN prediction errorMISR prediction benefitMISR real benefitMISR prediction error
Case 12068.982268.22199.242232.382278.446.02
Case 22066.362279.12212.762224.892236.2711.38
Case 32036.592089.1452.552238.262142.88?95.38
Case 42076.252277.07200.822207.92298.5890.68
Case 52040.762172.62131.862192.52158.91?33.59
Case 62065.552186.73121.182243.262291.4148.15
Case 72034.072177.14143.072165.762187.6921.93
Case 82041.772247.44205.672200.912244.6543.74
Case 92048.192229.03180.842155.812246.6390.82
Case 102051.722187.32135.62203.242204.421.18
Mean2053.0242211.383158.362206.4912228.98448.28
Tab.9  
Fig.10  
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