Generation of coherent blue light via bichromatic pumping in cesium vapor
Guiyuan Ge1, Li Tian1, Guoqing Zhang1, Ningxuan Zheng1, Wenliang Liu1,2, Vladimir Sovkov1,3, Jizhou Wu1,2,5(), Yuqing Li1,2, Yongming Fu4, Peng Li4, Jie Ma1,2,5(), Liantuan Xiao1,2, Suotang Jia1,2
1. State Key Laboratory of Quantum Optics and Quantum Optics Devices, Institute of Laser Spectroscopy, Shanxi University, Taiyuan 030006, China 2. Collaborative Innovation Center of Extreme Optics, Shanxi University, Taiyuan 030006, China 3. St. Petersburg State University, 7/9 Universitetskaya nab., St. Petersburg 199034, Russia 4. College of Physics and Electronic Engineering, Shanxi University, Taiyuan 030006, China 5. Hefei National Laboratory, Hefei 230088, China
Diode-pumped alkali lasers, possessing high efficiency and narrow linewidth, can provide feasible solutions for wavelength ranges difficult to reach by commercial lasers. In this study, we investigate a generation of coherent blue light (CBL) via four-wave mixing (FWM)-based up-conversion processes in cesium (Cs) vapor. A bichromatic pumping scheme with 852- and 917-nm lasers drives the Cs atoms to the 6D5/2 excited level, followed by cascaded decay of 6D5/2 → 7P3/2 → 6S1/2, producing 456-nm CBL under phase matching conditions. The fluorescence in multiple bands from blue to near- and far-infrared in the FWM process is demonstrated under different experimental conditions. To optimize the experimental parameters, we investigate the dependence of 456-nm CBL on the vapor temperature, frequency, and intensity of the two pump lasers. A maximum power of 2.94 mW is achieved with pump powers of 430 mW (for 852 nm) and 470 mW (for 917 nm). The corresponding conversion efficiency is 1.5%/W, three-fold higher than those in previous studies. Our results can contribute to fundamental research on atom−photon interactions and quantum metrology.
D. Xu D. , Chen F. , Guo J. , Z. Shao M. , J. Xie J. . Investigation on 447.3 nm blue-violet laser by extra-cavity frequency doubling of a diode-pumped cesium vapor laser. Opt. Laser Technol., 2016, 83(83): 119 https://doi.org/10.1016/j.optlastec.2016.04.003
2
V. Zhdanov B. , Venus G. , Smirnov V. , Glebov L. , J. Knize R. . Continuous wave Cs diode pumped alkali laser pumped by single emitter narrowband laser diode. Rev. Sci. Instrum., 2015, 86(8): 083104 https://doi.org/10.1063/1.4926883
3
V. Zhdanov B. , Ehrenreich T. , J. Knize R. . Highly efficient optically pumped cesium vapor laser. Opt. Commun., 2006, 260(2): 696 https://doi.org/10.1016/j.optcom.2005.11.042
4
F. Krupke W. , J. Beach R. , K. Kanz V. , A. Payne S. . Resonance transition 795-nm rubidium laser. Opt. Lett., 2003, 28(23): 2336 https://doi.org/10.1364/OL.28.002336
5
Akulshin A. , Budker D. , McLean R. . Directional infrared emission resulting from cascade population inversion and four-wave mixing in Rb vapor. Opt. Lett., 2014, 39(4): 845 https://doi.org/10.1364/OL.39.000845
6
F. Offer R. , W. C. Conway J. , Riis E. , Franke-Arnold S. , S. Arnold A. . Cavity-enhanced frequency up-conversion in rubidium vapor. Opt. Lett., 2016, 41(10): 2177 https://doi.org/10.1364/OL.41.002177
7
Gai B. , Liu J. , Wang P. , Chen Y. , Hu S. , Guo J. . Terahertz emitting and four wave mixing details in 6P3/2→11DJ pumped cesium vapor. J. Quant. Spectrosc. Radiat. Transf., 2021, 258: 107351 https://doi.org/10.1016/j.jqsrt.2020.107351
8
Gai B. , Hu S. , Chu J. , Wang P. , Cai X. , Guo J. . Collimated ultraviolet light generated by four-wave mixing process in Cs vapor. OSA Continuum, 2021, 4(9): 2410 https://doi.org/10.1364/OSAC.435249
9
Asano K. , Tsukamoto M. , Sechi Y. , Sato Y. , I. Masuno S. , Higashino R. , Hara T. , Sengoku M. , Yoshida M. . Laser metal deposition of pure copper on stainless steel with blue and IR diode lasers. Opt. Laser Technol., 2018, 107(1): 291 https://doi.org/10.1016/j.optlastec.2018.06.012
10
Lu G. , Sakamoto T. , Kawanishi T. . Wavelength conversion of optical 64QAM through FWM in HNLF and its performance optimization by constellation monitoring. Opt. Express, 2014, 22(1): 15 https://doi.org/10.1364/OE.22.000015
11
Stan-Sion C. , Enachescu M. , R. Petre A. , Duma M. , G. Ghita D. , Kizane G. , Baumane L. , Gabrusenoks J. , Halitovs M. , Avotina L. , Zarins A. , Likonen J. , Koivuranta S. , Kiisk M. . Comparison of tritium measurement techniques for a laser cleaned JET tile. Fusion Eng. Des., 2014, 89(11): 2628 https://doi.org/10.1016/j.fusengdes.2014.06.021
12
Markowski K. , Chorchos Ł. , P. Turkiewicz J. . Influence of four-wave mixing in short- and medium-range 1310 nm dense wavelength division multiplexing systems. Appl. Opt., 2016, 55(11): 3051 https://doi.org/10.1364/AO.55.003051
13
Ali F. , Muhammad F. , Habib U. , Khan Y. , Usman M. . Modeling and minimization of FWM effects in DWDM-based long-haul optical communication systems. Photonic Netw. Commun., 2021, 41(1): 36 https://doi.org/10.1007/s11107-020-00913-9
14
Zhang Y. , Zhang F. , Bian Y. . Application of laser communication in submarine communication. Opt. Commun. Tech., 2006, 30(7): 43
15
T. Schultz J. , Abend S. , Doring D. , E. Debs J. , A. Altin P. , D. White J. , P. Robins N. , D. Close J. . Coherent 455 nm beam production in a cesium vapor. Opt. Lett., 2009, 34(15): 2321 https://doi.org/10.1364/OL.34.002321
16
Akulshin A. , Pedreros Bustos F. , Budker D. . Intensity-correlated spiking of infrared and ultraviolet emission from sodium vapors. Opt. Lett., 2021, 46(9): 2131 https://doi.org/10.1364/OL.421409
17
S. Heavens O. . Radiative transition probabilities of the lower excited states of the alkali metals. J. Opt. Soc. Am., 1961, 51(10): 1058 https://doi.org/10.1364/JOSA.51.001058
18
Wu J. , Guo M. , Zhou H. , Liu J. , Li J. , Zhang J. . Experimental realization of efficient nondegenerate four-wave mixing in cesium atoms. Opt. Express, 2022, 30(8): 12576 https://doi.org/10.1364/OE.452790
19
J. Lee M. , H. Chen Chen , C. Wang Y. , A. Yu Wang . EIT-based all-optical switching and cross-phase modulation under the influence of four-wave mixing. Opt. Express, 2012, 20(10): 11057 https://doi.org/10.1364/OE.20.011057
20
Weeks T. , Wachsmann-Hogiu S. , Huser T. . Raman microscopy based on doubly-resonant four-wave mixing (DR-FWM). Opt. Express, 2009, 17(19): 17044 https://doi.org/10.1364/OE.17.017044
21
Wang G. , Cen L. , Qu Y. , Xue Y. , H. Wu J. , Y. Gao J. . Intensity-dependent effects on four-wave mixing based on electromagnetically induced transparency. Opt. Express, 2011, 19(22): 21614 https://doi.org/10.1364/OE.19.021614
22
Yan M. , G. Rickey E. , Zhu Y. . Suppression of two-photon absorption by quantum interference. Phys. Rev. A, 2001, 64(4): 043807 https://doi.org/10.1103/PhysRevA.64.043807
Y. Zhang Y. , Z. Wu J. , Y. He Y. , Zhang Y. , D. Hu Y. , X. Zhang J. , Y. Zhu S. . Observation of the interplay between seeded and self-seeded nondegenerate four-wave mixing in cesium vapor. Opt. Express, 2020, 28(12): 17723 https://doi.org/10.1364/OE.393032
25
Z. Wu J. , H. Xu Y. , G. Dong R. , X. Zhang J. . Experimental realization of wavelength multiplexed nonlinear upconversion in cesium atoms. Opt. Lett., 2021, 46(13): 3119 https://doi.org/10.1364/OL.428307
26
M. Akulshin A. , J. McLean R. , I. Sidorov A. , Hannaford P. . Collimated blue light generated by four-wave mixing in Rb vapour. Opt. Express, 2009, 17(25): 22861 https://doi.org/10.1364/OE.17.022861
27
Vernier A. , Franke-Arnold S. , Riis E. , S. Arnold A. . Enhanced frequency up-conversion in Rb vapor. Opt. Express, 2010, 18(16): 17020 https://doi.org/10.1364/OE.18.017020
28
P. Yuan J. , Liu H. , R. Wang L. , T. Xiao L. , T. Jia S. . Coherent 420 nm light generated by the cavity-enhanced four-wave mixing process in Rb vapor. Opt. Express, 2021, 29(4): 4858 https://doi.org/10.1364/OE.416307
29
Lam M. , B. Pal S. , Vogt T. , Kiffner M. , H. Li W. . Directional THz generation in hot Rb vapor excited to a Rydberg state. Opt. Lett., 2021, 46(5): 1017 https://doi.org/10.1364/OL.418618
30
Meijer T. , D. White J. , Smeets B. , Jeppesen M. , E. Scholten R. . Blue five-level frequency-upconversion system in rubidium. Opt. Lett., 2006, 31(7): 1002 https://doi.org/10.1364/OL.31.001002
31
Brekke E. , Potier S. . Optical cavity for enhanced parametric four-wave mixing in rubidium. Appl. Opt., 2017, 56(1): 46 https://doi.org/10.1364/AO.56.000046
32
F. Sell J. , A. Gearba M. , D. DePaola B. , J. Knize R. . Collimated blue and infrared beams generated by two-photon excitation in Rb vapor. Opt. Lett., 2014, 39(3): 528 https://doi.org/10.1364/OL.39.000528
33
Z. Wu J. , J. Guo M. , T. Zhou H. , H. Liu J. , H. Li J. , X. Zhang J. . Experimental realization of efficient nondegenerate four-wave mixing in cesium atoms. Opt. Express, 2022, 30(8): 12576 https://doi.org/10.1364/OE.452790
34
Ohtsuka T. , Nishimiya N. , Fukuda T. , Suzuki M. . Doppler-free two-photon spectroscopy of 6S1/2−6D3/2,5/2 transition in cesium. J. Phys. Soc. Jpn., 2005, 74(9): 2487 https://doi.org/10.1143/JPSJ.74.2487
35
Zhang Y. , W. Brown A. , Gan C. , Xiao M. . Intermixing between four-wave mixing and six-wave mixing in a four-level atomic system. J. Phys. At. Mol. Opt. Phys., 2007, 40(17): 3319 https://doi.org/10.1088/0953-4075/40/17/001
36
G. Joneckis L. , H. Shapiro J. . Quantum propagation in a Kerr medium: Lossless, dispersionless fiber. J. Opt. Soc. Am. B, 1994, 11(1): 150 https://doi.org/10.1364/JOSAB.11.000150
Matsuura M. , Kishi N. . High-speed wavelength conversion of RZ-DPSK signal using FWM in a quantum-dot SOA. IEEE Photonics Technol. Lett., 2011, 23(10): 615 https://doi.org/10.1109/LPT.2011.2119396
39
Ramírez-Martínez F. , Ponciano-Ojeda F. , Hernández-Gómez S. , Del Angel A. , Mojica-Casique C. , M. Hoyos-Campo L. , Flores-Mijangos J. , Sahagún D. , Jáuregui R. , Jiménez-Mier J. . Electric-dipole forbidden transitions for probing atomic state preparation: The case of the Autler–Townes effect. J. Phys. At. Mol. Opt. Phys., 2021, 54(9): 095002 https://doi.org/10.1088/1361-6455/abf156
40
A. Chan E. , A. Aljunid S. , I. Zheludev N. , Wilkowski D. , Ducloy M. . Doopler-free approach to optical pumping dynamics in the 6S1/2−5D5/2 electric quadrupole transition of cesium vapor. Opt. Lett., 2016, 41(9): 2005 https://doi.org/10.1364/OL.41.002005
41
Akulshin A. , Perrella C. , Truong G. , McLean R. , Luiten A. . Frequency evaluation of collimated blue light generated by wave mixing in Rb vapour. J. Phys. At. Mol. Opt. Phys., 2012, 45(24): 245503 https://doi.org/10.1088/0953-4075/45/24/245503
42
Brekke E. , Swan N. . Saturation and alternate pathways in four-wave mixing in rubidium. J. Opt. Soc. Am. B, 2019, 36(2): 421 https://doi.org/10.1364/JOSAB.36.000421
43
K. Wunderlich R. , R. Garrett W. , C. Hart R. , A. Moore M. , G. Payne M. . Nonlinear optical processes near the sodium 4D two-photon resonance. Phys. Rev. A, 1990, 41(11): 6345 https://doi.org/10.1103/PhysRevA.41.6345
44
A. Steck D., Webpage: steck.us/alkalidata, Revision 2.1.6, 20 September, 2013
45
P. Moreno M. , A. C. de Almeida A. , S. Vianna S. . Interference effect and Autler–Townes splitting in coherent blue light generated by four-wave mixing. Phys. Rev. A, 2019, 99(4): 043410 https://doi.org/10.1103/PhysRevA.99.043410