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Frontiers of Environmental Science & Engineering

ISSN 2095-2201

ISSN 2095-221X(Online)

CN 10-1013/X

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2018 Impact Factor: 3.883

Front. Environ. Sci. Eng.    2023, Vol. 17 Issue (11) : 131    https://doi.org/10.1007/s11783-023-1731-z
RESEARCH ARTICLE
Numerical modeling and performance evaluation of passive convergence-permeable reactive barrier (PC-PRB)
Kaixuan Zheng1, Dong Xie1, Yiqi Tan1, Zhenjiang Zhuo1, Tan Chen2, Hongtao Wang1(), Ying Yuan3(), Junlong Huang1, Tianwei Sun1, Fangming Xu1, Yuecen Dong1, Ximing Liang1
1. School of Environment, Tsinghua University, Beijing 100084, China
2. College of Life and Environmental Sciences, Minzu University of China, Beijing 100081, China
3. State Key Laboratory of Environmental Criteria and Risk Assessment, Chinese Research Academy of Environmental Sciences, Beijing 100012, China
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Abstract

● A 2D finite-element solute transport model, PRB-Trans, is developed.

● PC-PRB can significantly improve the remediation efficiency of PRB.

● PC-PRB can considerably reduce the required PRB dimensions and materials costs.

● The required PRB length decreases with the increase of pipe length, L p.

The passive convergence-permeable reactive barrier (PC-PRB) was proposed to address the limitations of traditional PRB configurations. To evaluate the hydraulic and pollutant removal performance of the PC-PRB system, we developed a simulation code named PRB-Trans. This code uses the two-dimensional (2D) finite element method to simulate groundwater flow and solute transport. Case studies demonstrate that PC-PRB technology is more efficient and cost-effective than continuous permeable reactive barrier (C-PRB) in treating the same contaminated plume. Implementation of PC-PRB technology results in a 33.3% and 72.7% reduction in PRB length (LPRB) and height (HPRB), respectively, while increasing 2D horizontal and 2D vertical pollutant treatment efficiencies of PRB by 87.8% and 266.8%, respectively. In addition, the PC-PRB technology has the ability to homogenize the pollutant concentration and pollutant flux through the PRB system, which can mitigate the problems arising from uneven distribution of pollutants in the C-PRB to some extent. The LPRB required for PC-PRB decreases as the water pipe length (Lp) increases, while the HPRB required initially decreases and then increases with increasing Lp. The effect of passive well height (Hw) on HPRB is not as significant as that of Lp on HPRB. Overall, PC-PRB presents a promising and advantageous PRB configuration in the effective treatment of various types of contaminated plumes.

Keywords Passive convergence-permeable reactive barrier      Numerical modeling      Hydraulic behavior assessment      Pollutant treatment performance evaluation      Influential factors analysis     
Corresponding Author(s): Hongtao Wang,Ying Yuan   
Issue Date: 15 November 2023
 Cite this article:   
Kaixuan Zheng,Dong Xie,Yiqi Tan, et al. Numerical modeling and performance evaluation of passive convergence-permeable reactive barrier (PC-PRB)[J]. Front. Environ. Sci. Eng., 2023, 17(11): 131.
 URL:  
https://academic.hep.com.cn/fese/EN/10.1007/s11783-023-1731-z
https://academic.hep.com.cn/fese/EN/Y2023/V17/I11/131
Fig.1  A schematic diagram of the PC-PRB system (Zheng et al., 2022b).
Fig.2  Representation of the main PC-PRB design parameters in the PRB-Trans code. (a) The horizontal 2D confined aquifer, (b) the vertical 2D confined aquifer.
ParametersValues (m)
PC-PRBPassive wellWell diameter, Dw5.0
Well height, Hw5.0
Water pipePipe length, Lp30.0
Pipe diameter, Dp1.0
Buried depth, Bp0.5
Buffer layerLayer thickness, Tb1.0
PRB systemPRB Length, LPRB36.0
PRB Thickness, TPRB3.0
PRB Height, HPRB6.0
C-PRBPRB Length, LPRB54.0
PRB Thickness, TPRB3.0
PRB Height, HPRB22.0
Tab.1  Geometric parameters and their values of the PC-PRB and C-PRB
Evaluation indicatorsDefinitionEstimation method
LPRB, HPRBPRB length/height required to completely intercept the contaminated plumeSolute transport module in PRB-Trans code
QMass of groundwater entering the PRB per unit timeZone water budget module in PRB-Trans code
qMass of groundwater entering the unit length/height of PRB per unit timeq=Q/LPRB
WWidth of the groundwater area that passes through rather than bypasses the PRBParticle tracer module in PRB-Trans code
wHydraulic capture width per unit PRB lengthw=W/LPRB
tContact time between pollutants and reactive materials in PRBt=TPRB·n·LPRB/Q
CAverage concentration of ammonia nitrogen in contaminated groundwater via PRBSolute transport module in PRB-Trans code
FMass of ammonia nitrogen entering the PRB per unit timeF=C·Q
fMass of ammonia nitrogen entering the unit PRB length per unit timef=F/LPRB
Tab.2  Definitions and estimation methods of the performance evaluation indicators
Fig.3  Comparison of pollutant concentration distribution in plumes treated with PC-PRB and C-PRB. (a) The horizontal 2D pollutant concentration distribution of plume treated with C-PRB (LPRB = 54 m), (b) the horizontal 2D pollutant concentration distribution of plume treated with PC-PRB (LPRB = 36 m), (c) the vertical 2D pollutant concentration distribution of plume treated with C-PRB (HPRB = 22 m), and (d) the vertical 2D pollutant concentration distribution of plume treated with PC-PRB (HPRB = 6 m).
IndicatorsConfigurationZone ⅠZone ⅡZone ⅢTotalMean
LPRB (m)C-PRB18.018.018.054.0
PC-PRB12.012.012.036.0
ΔLPRB (%)?33.33?33.33?33.33?33.33
Qh (m3/d)C-PRB0.1880.1900.2070.585
PC-PRB0.1980.1970.1980.594
ΔQ (%)5.33.7?4.31.5
qh (m3/(m·d))C-PRB0.0100.0110.0120.011
PC-PRB0.0170.0160.0170.017
Δq (%)65.049.238.252.3
Wh (m)C-PRB59.0
PC-PRB57.0
ΔW (%)?3.4
wh (m)C-PRB1.093
PC-PRB1.583
Δw (%)44.8
th (d)C-PRB40.21339.78936.52238.769
PC-PRB25.45525.58425.32725.455
Δt (%)?36.7?35.7?30.7?34.3
Ch (mg/L)C-PRB35.77230.79022.48329.681
PC-PRB39.68636.82833.30736.607
ΔC (%)10.919.648.123.3
Fh (g/d)C-PRB6.7255.8504.65417.364
PC-PRB7.8587.2556.62821.745
ΔF (%)16.84524.01942.41525.231
fh (g/(m·d))PRB0.3740.3250.2590.322
PC-PRB0.6550.6050.5520.604
Δf (%)75.386.0113.687.8
Tab.3  Comparison between the horizontal 2D performance evaluation indicators of the PC-PRB and those of the PRB (at t = 3000 d)
IndicatorsConfigurationZone ⅠZone ⅡTotalMean
HPRB (m)C-PRB11.011.022.0
PC-PRB3.03.06.0
ΔH (%)?72.7?72.7?72.7
Qv (m3/d)C-PRB0.1140.1230.237
PC-PRB0.0870.0870.174
ΔQ (%)?23.7?29.3?26.6
qv (m3/(m·d))C-PRB0.0100.0110.011
PC-PRB0.0290.0290.029
Δq (%)190.0163.6163.6
Wv (m)C-PRB24.0
PC-PRB17.0
ΔW (%)?29.2
wv (m)C-PRB1.091
PC-PRB2.833
Δw (%)159.7
tv (d)C-PRB40.52637.56138.987
PC-PRB14.48314.48314.483
Δt (%)?64.3?61.4?62.9
Cv (mg/L)C-PRB21.78728.13824.962
PC-PRB34.60033.43334.017
ΔC (%)58.818.836.3
Fv (g/d)C-PRB2.4843.4615.916
PC-PRB3.0102.9095.919
ΔF (%)21.2?16.00.0
fv (g/(m·d))C-PRB0.2260.3150.269
PC-PRB1.0030.9700.986
Δf (%)344.4208.2266.8
Tab.4  Comparison between the vertical 2D performance evaluation indicator of the PC-PRB and those of the PRB (at t = 3000 d)
Fig.4  Effect of Lp at three width levels of plumes on: (a) ΔLPRB, (b) ΔQh, (c) ΔWh, (d) ΔFh, (e) ΔCh, (f) Δqh, (g) Δwh, (h) Δfh, (i) Δth.
Fig.5  Effect of Lp at three depth levels of plumes on: (a) ΔHPRB, (b) ΔQv, (c) ΔWv, (d) ΔFv, (e) ΔCv, (f) Δqv, (g) Δwv, (h) Δfv, (i) Δtv.
Fig.6  Effect of Hw at three depth levels of plumes on: (a) ΔHPRB, (b) ΔQv, (c) ΔWv, (d) ΔFv, (e) ΔCv, (f) Δqv, (g) Δwv, (h) Δfv, (i) Δtv.
1 A F Ali , Z T Abd Ali . (2020). Sustainable use of concrete demolition waste as reactive material in permeable barrier for remediation of groundwater: batch and continuous study. Journal of Environmental Engineering, 146(7): 04020048
https://doi.org/10.1061/(ASCE)EE.1943-7870.0001714
2 I Bortone , S Chianese , A Erto , A Di Nardo , C De Crescenzo , D Karatza , G F Santonastaso , D Musmarra . (2019). An optimized configuration of adsorptive wells for the remediation of an aquifer contaminated by multiple aromatic hydrocarbon pollutants. Science of the Total Environment, 696: 133731
https://doi.org/10.1016/j.scitotenv.2019.133731
3 I Bortone , A Di Nardo , M Di Natale , A Erto , D Musmarra , G Santonastaso . (2013). Remediation of an aquifer polluted with dissolved tetrachloroethylene by an array of wells filled with activated carbon. Journal of Hazardous Materials, 260: 914–920
https://doi.org/10.1016/j.jhazmat.2013.06.050
4 I Bortone , A Erto , G Santonastaso , A Di Nardo , M Di Natale , D Musmarra . (2015). Design of Permeable Adsorptive Barriers (PABs) for groundwater remediation by COMSOL multi-physics simulations. Desalination and Water Treatment, 55(12): 3231–3240
https://doi.org/10.1080/19443994.2014.957931
5 Y Cheng , Y Shan , Y Xue , Y Zhu , X Wang , L Xue , Y Liu , F Qiao , M Zhang . (2022). Variation characteristics of atmospheric methane and carbon dioxide in summertime at a coastal site in the South China Sea. Frontiers of Environmental Science & Engineering, 16(11): 139
https://doi.org/10.1007/s11783-022-1574-z
6 B Courcelles . (2015). Guidelines for preliminary design of funnel-and-gate reactive barriers. International Journal of Environment and Pollution Remediation, 3(1): 16–26
7 R Elder Carl , H Benson Craig . (2019). Performance and economic comparison of PRB types in heterogeneous aquifers. Environmental Geotechnics, 6(4): 214–224
https://doi.org/10.1680/jenge.17.00063
8 A Faisal , A Sulaymon , Q Khaliefa . (2018). A review of permeable reactive barrier as passive sustainable technology for groundwater remediation. International Journal of Environmental Science and Technology, 15(5): 1123–1138
https://doi.org/10.1007/s13762-017-1466-0
9 P P Falciglia , E Gagliano , V Brancato , G Malandrino , G Finocchiaro , A Catalfo , G De Guidi , S Romano , P Roccaro , F G Vagliasindi . (2020). Microwave based regenerating permeable reactive barriers (MW-PRBs): proof of concept and application for Cs removal. Chemosphere, 251: 126582
https://doi.org/10.1016/j.chemosphere.2020.126582
10 A R (1999) Gavaskar. Design and construction techniques for permeable reactive barriers. Journal of Hazardous Materials, 68(1-2): 41-71
11 R W GillhamJ VoganL GuiM DucheneJ (2010) Son. Iron barrier walls for chlorinated solvent remediation. In: Stroo H F, Ward C H, eds. In situ Remediation of Chlorinated Solvent Plumes. New York: Springer, 537–571
12 N GuptaT C (1999) Fox. Hydrogeologic modeling for permeable reactive barriers. Journal of Hazardous Materials, 68(1–2): 19–39
13 M R Higgins , T M Olson . (2009). Life-cycle case study comparison of permeable reactive barrier versus pump-and-treat remediation. Environmental Science & Technology, 43(24): 9432–9438
https://doi.org/10.1021/es9015537
14 Y Jiang , B Xi , R Li , M Li , Z Xu , Y Yang , S Gao . (2019). Advances in Fe (III) bioreduction and its application prospect for groundwater remediation: a review. Frontiers of Environmental Science & Engineering, 13(6): 89
https://doi.org/10.1007/s11783-019-1173-9
15 M Kheirandish , C An , Z Chen , X Geng , M Boufadel . (2022). Numerical simulation of benzene transport in shoreline groundwater affected by tides under different conditions. Frontiers of Environmental Science & Engineering, 16(5): 61
https://doi.org/10.1007/s11783-022-1540-9
16 Y Li , Y Huang , W Wu , M Yan , Y Xie . (2021). Research and application of arsenic-contaminated groundwater remediation by manganese ore permeable reactive barrier. Environmental Technology, 42(13): 2009–2020
https://doi.org/10.1080/09593330.2019.1687587
17 S Liu , X Li , H Wang . (2011). Hydraulics analysis for groundwater flow through permeable reactive barriers. Environmental Modeling and Assessment, 16(6): 591–598
https://doi.org/10.1007/s10666-011-9268-0
18 X Lu , M Li , H Deng , P Lin , M R Matsumoto , X Liu . (2016). Application of electrochemical depassivation in PRB systems to recovery Fe0 reactivity. Frontiers of Environmental Science & Engineering, 10(4): 4
https://doi.org/10.1007/s11783-016-0843-0
19 I Maamoun , O Eljamal , O Falyouna , R Eljamal , Y Sugihara . (2020). Multi-objective optimization of permeable reactive barrier design for Cr(VI) removal from groundwater. Ecotoxicology and Environmental Safety, 200: 110773
https://doi.org/10.1016/j.ecoenv.2020.110773
20 F Obiri-Nyarko , S J Grajales-Mesa , G Malina . (2014). An overview of permeable reactive barriers for in situ sustainable groundwater remediation. Chemosphere, 111: 243–259
https://doi.org/10.1016/j.chemosphere.2014.03.112
21 B D (2005) Painter. Optimisation of Permeable Reactive Barrier Systems for the Remediation of Contaminated Groundwater. Dissertation for the Doctoral Degree. Lincoln: Lincoln University
22 Phillips D (2009). Permeable reactive barriers: a sustainable technology for cleaning contaminated groundwater in developing countries. Desalination, 248(1−3): 352−359
23 G SantonastasoI BortoneS ChianeseA ErtoNardo A DiNatale M DiD (2016) Musmarra. Application of a discontinuous permeable adsorptive barrier for aquifer remediation: a comparison with a continuous adsorptive barrier. Desalination and Water Treatment, 57(48–49): 248–491
24 G F Santonastaso , I Bortone , S Chianese , A Di Nardo , M Di Natale , A Erto , D Karatza , D Musmarra . (2018). Discontinuous permeable adsorptive barrier design and cost analysis: a methodological approach to optimisation. Environmental Science and Pollution Research International, 25(27): 26793–26800
https://doi.org/10.1007/s11356-017-0220-y
25 K Song , S Zhu , Y Lu , G Dao , Y Wu , Z Chen , S Wang , J Liu , W Zhou , H Hu . (2022). Modelling the thresholds of nitrogen/phosphorus concentration and hydraulic retention time for bloom control in reclaimed water landscape. Frontiers of Environmental Science & Engineering, 16(10): 129
https://doi.org/10.1007/s11783-022-1564-1
26 A K Thakur , M Vithanage , D B Das , M Kumar . (2020). A review on design, material selection, mechanism, and modelling of permeable reactive barrier for community-scale groundwater treatment. Environmental Technology & Innovation, 19: 100917
https://doi.org/10.1016/j.eti.2020.100917
27 R Thiruvenkatachari , S Vigneswaran , R Naidu . (2008). Permeable reactive barrier for groundwater remediation. Journal of Industrial and Engineering Chemistry, 14(2): 145–156
https://doi.org/10.1016/j.jiec.2007.10.001
28 M Torregrosa , A Schwarz , I Nancucheo , E Balladares . (2019). Evaluation of the bio-protection mechanism in diffusive exchange permeable reactive barriers for the treatment of acid mine drainage. Science of the Total Environment, 655: 374–383
https://doi.org/10.1016/j.scitotenv.2018.11.083
29 N VanStone , A Przepiora , J Vogan , G Lacrampe-Couloume , B Powers , E Perez , S Mabury , B Sherwood Lollar . (2005). Monitoring trichloroethene remediation at an iron permeable reactive barrier using stable carbon isotopic analysis. Journal of Contaminant Hydrology, 78(4): 313–325
https://doi.org/10.1016/j.jconhyd.2005.05.013
30 V R Vermeul , J E Szecsody , B G Fritz , M D Williams , R C Moore , J S Fruchter . (2014). An injectable apatite permeable reactive barrier for in situ 90Sr immobilization. Ground Water Monitoring and Remediation, 34(2): 28–41
https://doi.org/10.1111/gwmr.12055
31 H Wan , J Bian , H Zhang , Y Li . (2021). Assessment of future climate change impacts on water-heat-salt migration in unsaturated frozen soil using CoupModel. Frontiers of Environmental Science & Engineering, 15(1): 10
https://doi.org/10.1007/s11783-020-1302-5
32 R D Wilson , D M Mackay , J A Cherry . (1997). Arrays of unpumped wells for plume migration control by semi-passive in situ remediation. Ground Water Monitoring and Remediation, 17(3): 185–193
https://doi.org/10.1111/j.1745-6592.1997.tb00594.x
33 Z Yin , Q Lin , S Xu . (2021). Using hydrochemical signatures to characterize the long-period evolution of groundwater information in the Dagu River Basin, China. Frontiers of Environmental Science & Engineering, 15(5): 105
https://doi.org/10.1007/s11783-021-1393-7
34 R Zhang , H Sun , J Yin . (2008). Arsenic and chromate removal from water by iron chips: effects of anions. Frontiers of Environmental Science & Engineering in China, 2(2): 203–208
https://doi.org/10.1007/s11783-008-0036-6
35 B Zhao , Z Sun , Y Liu . (2022). An overview of in-situ remediation for nitrate in groundwater. Science of the Total Environment, 804: 149981
https://doi.org/10.1016/j.scitotenv.2021.149981
36 K ZhengJ HuangX LuoH WangT (2022a) Chen. Application progress of numerical simulation in permeable reactive barrier engineering design. Environmental Engineering, 40(6): 22–30 (in Chinese)
37 K Zheng , X Luo , Y Tan , Z Li , H Wang , T Chen , L Zhao , L Zhan . (2022b). Passive convergence-permeable reactive barrier (PC-PRB): an effective configuration to enhance hydraulic performance. Frontiers of Environmental Science & Engineering, 16(12): 156
https://doi.org/10.1007/s11783-022-1591-y
[1] FSE-23026-OF-ZKX_suppl_1 Download
[1] Kaixuan Zheng, Xingshen Luo, Yiqi Tan, Zhonglei Li, Hongtao Wang, Tan Chen, Li Zhao, Liangtong Zhan. Passive convergence-permeable reactive barrier (PC-PRB): An effective configuration to enhance hydraulic performance[J]. Front. Environ. Sci. Eng., 2022, 16(12): 156-.
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