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Frontiers of Environmental Science & Engineering

ISSN 2095-2201

ISSN 2095-221X(Online)

CN 10-1013/X

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2018 Impact Factor: 3.883

Front. Environ. Sci. Eng.    2021, Vol. 15 Issue (6) : 140    https://doi.org/10.1007/s11783-021-1434-2
RESEARCH ARTICLE
Local and regional contributions to PM2.5 in the Beijing 2022 Winter Olympics infrastructure areas during haze episodes
Yue Wang, Mengshuang Shi, Zhaofeng Lv, Huan Liu(), Kebin He
State Key Joint Laboratory of ESPC, State Environmental Protection Key Laboratory of Sources and Control of Air Pollution Complex, International Joint Laboratory on Low Carbon Clean Energy Innovation, School of the Environment, Tsinghua University, Beijing 100084, China
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Abstract

• Regional transportation contributed more than local emissions during haze episodes.

• Short-range regional transportation contributed the most to the PM2.5 in the OIAs.

• Low wind speeds and low PBLHs led to higher local contributions to Beijing.

The 2022 Winter Olympics is scheduled to take place in Beijing and Zhangjiakou, which were defined as OIAs (Olympic infrastructure areas) in this study. This study presents the characteristics and source apportionment of PM2.5 in the OIAs, China. The entire region of mainland China, except for the OIAs, was divided into 9 source regions, including four regions in the BTH(Beijing-Tianjin-Hebei) region, the four provinces surrounding the BTH and the remaining areas. Using CAMx/PSAT, the contributions of the nine regions to the PM2.5 concentration in the OIAs were simulated spatially and temporally. The simulated source apportionment results showed that the contribution of regional transportation was 48.78%, and when PM2.5 concentration was larger than 75 μg/m3 central Hebei was the largest contributor with a contribution of 19.18%, followed by Tianjin, northern Hebei, Shanxi, Inner Mongolia, Shandong, southern Hebei, Henan and Liaoning. Furthermore, the contribution from neighboring regions of the OIAs was 47.12%, which was nearly twice that of long-range transportation. Haze episodes were analyzed, and the results presented the importance of regional transportation during severe PM2.5 pollution periods. It was also found that they were associated with differences in pollution sources between Zhangjiakou and Beijing. Regional transportation was the main factor affecting PM2.5 pollution in Zhangjiakou due to its low local emissions. Stagnant weather with a low planetary boundary layer height and a low wind velocity prevented the local emitted pollutants in Beijing from being transported outside, and as a result, local emissions constituted a larger contribution in Beijing.

Keywords 2022 Winter Olympics      PM2.5      Source apportionment     
Corresponding Author(s): Huan Liu   
Issue Date: 14 May 2021
 Cite this article:   
Yue Wang,Mengshuang Shi,Zhaofeng Lv, et al. Local and regional contributions to PM2.5 in the Beijing 2022 Winter Olympics infrastructure areas during haze episodes[J]. Front. Environ. Sci. Eng., 2021, 15(6): 140.
 URL:  
https://academic.hep.com.cn/fese/EN/10.1007/s11783-021-1434-2
https://academic.hep.com.cn/fese/EN/Y2021/V15/I6/140
City SIM MON Bias R RMSE NMB (%) NME (%) IOA MFB (%) MFE (%)
Beijing 90.57 88.45 0.76 0.69 72.16 ?7.91 47.36 0.8 10.61 58.95
Zhangjiakou 17.66 29.09 0.26 0.51 30.77 ?48.26 58.95 0.62 52.94 72.18
Tab.1  Evaluation of CAMx model performance
Fig.1  Comparison between the simulated and observed hourly concentration of PM2.5.
Fig.2  Monthly average concentration of PM2.5 for January, 2015.
Fig.3  Temporal variation of (a) contributions and (b) contribution percentage of different regions to PM2.5 concentration in OIA during January, 2015.
Fig.4  Average contribution percentage of different source regions under different PM2.5 concentration level.
Fig.5  Hourly variations in the proportion of PM2.5 components.
Fig.6  Daily variations in the contribution of regional transportation to different PM2.5 components (the sources emitted outside research area means regional transport-related contribution.TR-: regional transport-related contributions).
Region Primary PM2.5 Sulfate Nitrate Ammonium SOA
>75 ≤75 >75 ≤75 >75 ≤75 >75 ≤75 >75 ≤75
OIAs 46.38 63.73 22.18 43.22 16.9 41.35 40.63 59.06 31.55 57.32
TJ 7.2 3.46 9.44 3.77 10.57 4.37 5.49 2.56 13.04 5.26
NH 5.6 2.6 11.23 3.19 11.38 3.41 5.17 2.48 6.76 2.75
CH 19.72 9.01 16.1 7.64 18.78 10.31 20.04 8.08 18.01 8.55
SH 2.32 0.93 2.61 0.99 4.13 1.87 3.14 1.03 3.05 1.13
LN 1.22 0.17 2.24 0.29 2.73 0.4 1.21 0.15 1.68 0.19
IM 5.02 12.92 9.44 25.71 7.5 24.36 7.76 18.59 6 15.51
SX 5.6 5.05 11.84 9.65 7.09 6.66 5.72 5.1 5.57 4.67
HN 1.46 0.27 1.8 0.32 3.85 0.79 3.1 0.49 3.13 0.48
SD 3.39 0.85 5.74 1.28 8.98 2.35 4.96 1.04 7.7 1.6
Oth. 2.09 1.01 7.38 3.94 8.09 4.13 2.78 1.42 3.51 2.54
Tab.2  Contribution of regional transportation to PM2.5 and its components under different PM2.5 concentration level
1 J W Boylan, A G Russell (2006). PM and light extinction model performance metrics, goals, and criteria for three-dimensional air quality models. Atmospheric Environment, 40(26): 4946–4959
https://doi.org/10.1016/j.atmosenv.2005.09.087
2 X Chang, S Wang, B Zhao, J Xing, X Liu, L Wei, Y Song, W Wu, S Cai, H Zheng, D Ding, M Zheng (2019). Contributions of inter-city and regional transport to PM2.5 concentrations in the Beijing-Tianjin-Hebei region and its implications on regional joint air pollution control. Science of the Total Environment, 660: 1191–1200
https://doi.org/10.1016/j.scitotenv.2018.12.474
3 Y Chen, Y Zhou, X Zhao (2020). PM2.5 over North China based on MODIS AOD and effect of meteorological elements during 2003–2015. Frontiers of Environmental Science & Engineering, 14(2): 23
https://doi.org/10.1007/s11783-019-1202-8
4 N Fann, D Risley (2013). The public health context for PM2.5 and ozone air quality trends. Air Quality, Atmosphere & Health, 6(1): 1–11
https://doi.org/10.1007/s11869-010-0125-0
5 B R Gurjar, A Jain, A Sharma, A Agarwal, P Gupta, A S Nagpure, J Lelieveld (2010). Human health risks in megacities due to air pollution. Atmospheric Environment, 44(36): 4606–4613
https://doi.org/10.1016/j.atmosenv.2010.08.011
6 B J Huang(2014). Emission Inventory of Volatile Organic Compounds from Field Burning of Crop Residues in Hubei Province, China. Stafa-Zurich: Trans Tech Publications Ltd. Trans Tech Publ, 1280–1284
7 X Huang, Z Liu, J Liu, B Hu, T Wen, G Tang, J Zhang, F Wu, D Ji, L Wang, Y Wang (2017). Chemical characterization and synergetic source apportionment of PM2.5 at multiple sites in the Beijing-Tianjin-Hebei region, China. Atmospheric Chemistry and Physics, 17(21): 12941–12962
https://doi.org/10.5194/acp-2017-446
8 X Huang, Z Liu, J Zhang, T Wen, D Ji, Y Wang (2016). Seasonal variation and secondary formation of size-segregated aerosol water-soluble inorganic ions during pollution episodes in Beijing. Atmospheric Research, 168: 70–79
https://doi.org/10.1016/j.atmosres.2015.08.021
9 M J Kleeman, Q Ying, J Lu, M J Mysliwiec, R J Griffin, J Chen, S Clegg (2007). Source apportionment of secondary organic aerosol during a severe photochemical smog episode. Atmospheric Environment, 41(3): 576–591
https://doi.org/10.1016/j.atmosenv.2006.08.042
10 X Li, Y Wang, X Guo, Y Wang (2013). Seasonal variation and source apportionment of organic and inorganic compounds in PM2.5 and PM10 particulates in Beijing, China. Journal of Environmental Sciences (China), 25(4): 741–750
https://doi.org/10.1016/S1001-0742(12)60121-1
11 X Li, Q Zhang, Y Zhang, L Zhang, Y Wang, Q Zhang, M Li, Y Zheng, G Geng, T J Wallington, W Han, W Shen, K He (2017). Attribution of PM2.5 exposure in Beijing-Tianjin-Hebei region to emissions: Implication to control strategies. Science Bulletin, 62(13): 957–964
https://doi.org/10.1016/j.scib.2017.06.005
12 Y Lin, K Huang, G Zhuang, J S Fu, Q Wang, T Liu, C Deng, Q Fu (2014). A multi-year evolution of aerosol chemistry impacting visibility and haze formation over an Eastern Asia megacity, Shanghai. Atmospheric Environment, 92: 76–86
https://doi.org/10.1016/j.atmosenv.2014.04.007
13 Y C Lin, S C Hsu, C C K Chou, R Zhang, Y Wu, S J Kao, L Luo, C H Huang, S H Lin, Y T Huang (2016). Wintertime haze deterioration in Beijing by industrial pollution deduced from trace metal fingerprints and enhanced health risk by heavy metals. Environmental Pollution, 208: 284–293
https://doi.org/10.1016/j.envpol.2015.07.044
14 X Qiao, Q Ying, X Li, H Zhang, J Hu, Y Tang, X Chen (2018). Source apportionment of PM2.5 for 25 Chinese provincial capitals and municipalities using a source-oriented Community Multiscale Air Quality model. Science of the Total Environment, 612: 462–471
https://doi.org/10.1016/j.scitotenv.2017.08.272
15 J Quan, Q Zhang, H He, J Liu, M Huang, H Jin (2011). Analysis of the formation of fog and haze in North China Plain (NCP). Atmospheric Chemistry and Physics, 11(15): 8205–8214
https://doi.org/10.5194/acpd-11-11911-2011
16 G L Shi, X Li, Y C Feng, Y Q Wang, J H Wu, J Li, T Zhu (2009). Combined source apportionment, using positive matrix factorization-chemical mass balance and principal component analysis/multiple linear regression-chemical mass balance models. Atmospheric Environment, 43(18): 2929–2937
https://doi.org/10.1016/j.atmosenv.2009.02.054
17 K Skyllakou, B N Murphy, A G Megaritis, C Fountoukis, S N Pandis (2014). Contributions of local and regional sources to fine PM in the megacity of Paris. Atmospheric Chemistry and Physics, 14(5): 2343–2352
https://doi.org/10.5194/acpd-13-25769-2013
18 Y Sun, G Zhuang, A Tang, Y Wang, Z An (2006). Chemical characteristics of PM2.5 and PM10 in haze-fog episodes in Beijing. Environmental Science & Technology, 40(10): 3148–3155
https://doi.org/10.1021/es051533g
19 K M Wagstrom, S N Pandis, G Yarwood, G M Wilson, R E Morris (2008). Development and application of a computationally efficient particulate matter apportionment algorithm in a three-dimensional chemical transport model. Atmospheric Environment, 42(22): 5650–5659
https://doi.org/10.1016/j.atmosenv.2008.03.012
20 X Wang, W Wei, S Cheng, J Li, H Zhang, Z Lv (2018). Characteristics and classification of PM2.5 pollution episodes in Beijing from 2013 to 2015. Science of the Total Environment, 612: 170–179
https://doi.org/10.1016/j.scitotenv.2017.08.206
21 X S Wang, C Q Yan, S X Wang, Y J Zhang, J Cai, A G Russell, Y H Zhang, Y T Hu, M Zheng (2015a). Comparison and overview of PM2.5 source apportionment methods. Chinese Science Bulletin, 60(2): 109–121
https://doi.org/10.1360/N972014-00975
22 Y Wang, S Bao, S Wang, Y Hu, X Shi, J Wang, B Zhao, J Jiang, M Zheng, M Wu, A G Russell, Y Wang, J Hao (2017). Local and regional contributions to fine particulate matter in Beijing during heavy haze episodes. Science of the Total Environment, 580: 283–296
https://doi.org/10.1016/j.scitotenv.2016.12.127
23 W Wen, X Ma, P Wei, S Cheng, X Wang, X He, L Liu (2018). Understanding the regional transport contributions of primary and secondary PM2.5 components over Beijing during a severe pollution episodes. Aerosol and Air Quality Research, 18(7): 1720–1733
https://doi.org/10.4209/aaqr.2017.10.0406
24 T Xu, Y Song, M Liu, X Cai, H Zhang, J Guo, T Zhu (2019). Temperature inversions in severe polluted days derived from radiosonde data in North China from 2011 to 2016. Science of the Total Environment, 647: 1011–1020
https://doi.org/10.1016/j.scitotenv.2018.08.088
25 G Yarwood, S Rao, M Yocke, G Whitten (2005). Updates to the Carbon Bond chemical mechanism: CB05, Final Report Prepared for US EPA. Website:
26 H Zhang, S Cheng, J Li, S Yao, X Wang (2019a). Investigating the aerosol mass and chemical components characteristics and feedback effects on the meteorological factors in the Beijing-Tianjin-Hebei region, China. Environmental Pollution, 244: 495–502
27 H Zhang, S Cheng, S Yao, X Wang, J Zhang (2019b). Multiple perspectives for modeling regional PM2.5 transport across cities in the Beijing-Tianjin-Hebei region during haze episodes. Atmospheric Environment, 212: 22–35
https://doi.org/10.1016/j.atmosenv.2019.05.031
28 H Zhang, S P Denero, D K Joe, H H Lee, S H Chen, J Michalakes, M J Kleeman (2014). Development of a source oriented version of the WRF/Chem model and its application to the California regional PM10/PM2.5 air quality study. Atmospheric Chemistry and Physics, 14(1): 485–503
https://doi.org/10.5194/acpd-13-16457-2013
29 Y Zhang, B Zhu, J Gao, H Kang, P Yang, L Wang, J Zhang (2017). The source apportionment of primary PM2.5 in an aerosol pollution event over Beijing-Tianjin-Hebei region using WRF-Chem, China. Aerosol and Air Quality Research, 17(12): 2966–2980
https://doi.org/10.4209/aaqr.2016.10.0442
30 Z Y Zhang, M S Wong, K H Lee (2015b). Estimation of potential source regions of PM2.5 in Beijing using backward trajectories. Atmospheric Pollution Research, 6(1): 173–177
https://doi.org/10.5094/APR.2015.020
31 B Zhao, W Wu, S Wang, J Xing, X Chang, K N Liou, J H Jiang, Y Gu, C Jang, J S Fu, Y Zhu, J Wang, Y Lin, J Hao (2017). A modeling study of the nonlinear response of fine particles to air pollutant emissions in the Beijing-Tianjin-Hebei region. Atmospheric Chemistry and Physics, 17(19): 12031–12050
https://doi.org/10.5194/acp-17-12031-2017
32 B Zheng, Q Zhang, Y Zhang, K B He, K Wang, G J Zheng, F K Duan, Y L Ma, T Kimoto (2015). Heterogeneous chemistry: A mechanism missing in current models to explain secondary inorganic aerosol formation during the January 2013 haze episode in North China. Atmospheric Chemistry and Physics, 15(4): 2031–2049
https://doi.org/10.5194/acp-15-2031-2015
33 Y Zhou, X Xing, J Lang, D Chen, S Cheng, L Wei, X Wei, C Liu (2017). A comprehensive biomass burning emission inventory with high spatial and temporal resolution in China. Atmospheric Chemistry and Physics, 17(4): 2839–2864
https://doi.org/10.5194/acp-17-2839-2017
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