Effects of different sediment fractions on sorption of galaxolide

doi:10.1007/s11783-010-0259-1

Front Envir Sci Eng

2012, Vol. 6

Issue (1) : 59-65 https://doi.org/10.1007/s11783-010-0259-1

RESEARCH ARTICLE

Effects of different sediment fractions on sorption of galaxolide

Lixia JIN, Mengchang HE(

), Jinghuan ZHANG

State Key Laboratory of Water Environment Simulation, School of Environment, Beijing Normal University, Beijing 100875, China

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Abstract

Sorption isotherms of galaxolide (HHCB) of different fractions from two sediments with different mineral and organic carbon contents were determined to compare HHCB sorption behavior and contribution to the total sorption. The HHCB sorption isotherms that used the batch equilibration method were studied on different sediments of different fractions. The sorption isotherms of 600°C heating fractions were detailed using the linear model, while the other fractions were nonlinear and fitted well with the Freundlich model. The dissolved organic carbon (DOC) removed, NaOH extracted, and 375°C heating fractions showed more nonlinear sorption than the original sediments, which suggested more heterogeneous sorption sites in these fractions. Compared to the original sediments, the 375°C heating fractions had higher carbon-normalized distribution coefficient (K_oc) values, indicating a higher sorption affinity for HHCB. Among the different sediment fractions, the contribution of the 600°C heating fractions to the overall sorption were the lowest (<20%), while the 375°C heating fractions were the highest (up to 85%).

Keywords galaxolide (HHCB) sorption organic carbon sediment carbon-normalized distribution coefficient (K_oc)

Corresponding Author(s): HE Mengchang,Email:hemc@bnu.edu.cn

Issue Date: 01 February 2012

Cite this article:

Lixia JIN,Mengchang HE,Jinghuan ZHANG. Effects of different sediment fractions on sorption of galaxolide[J]. Front Envir Sci Eng, 2012, 6(1): 59-65.

URL:

https://academic.hep.com.cn/fese/EN/10.1007/s11783-010-0259-1
https://academic.hep.com.cn/fese/EN/Y2012/V6/I1/59

Tab.1 Characteristics of different fractions from two river sediments

Fig.1 FTIR spectra of different sediment fractions
Note: a and f- original sediment, b and g- DOC removed, c and h- NaOH extracted, d and i- heated at 375°C, and e and j- heated at 600°C

Fig.2 Sorption isotherms of HHCB on different sediment fractions

Tab.2 Fitting parameters by linear and Freundlich models for HHCB sorption on different fractions from two river sediments

Fig.3 Contribution of each fraction to total HHCB sorption by the original sediments

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