Catalytic combustion of volatile organic compounds using perovskite oxides catalysts—a review

doi:10.1007/s11705-023-2324-x

Front. Chem. Sci. Eng.

2023, Vol. 17

Issue (11) : 1649-1676 https://doi.org/10.1007/s11705-023-2324-x

REVIEW ARTICLE

Catalytic combustion of volatile organic compounds using perovskite oxides catalysts—a review

Shan Wang^1,², Ping Xiao², Jie Yang², Sónia A.C. Carabineiro³, Marek Wiśniewski⁴, Junjiang Zhu²(

), Xinying Liu^1,⁵(

)

¹. Institute for the Development of Energy for African Sustainability, College of Science, Engineering and Technology, University of South Africa, Johannesburg 1710, South Africa
². Hubei Key Laboratory of Biomass Fibers and Eco-dyeing & Finishing, College of Chemistry and Chemical Engineering, Wuhan Textile University, Wuhan 430200, China
³. LAQV-REQUIMTE, Department of Chemistry, NOVA School of Science and Technology, Universidade NOVA de Lisboa, 2829-516 Caparica, Portugal
⁴. Physicochemistry of Carbon Materials Research Group, Faculty of Chemistry, Nicolaus Copernicus University in Toruń, 87-100 Toruń, Poland
⁵. Zhijiang College of Zhejiang University of Technology, Shaoxing 312030, China

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Abstract

With the rapid development of industry, volatile organic compounds (VOCs) are gaining attention as a class of pollutants that need to be eliminated due to their adverse effects on the environment and human health. Catalytic combustion is the most popular technology used for the removal of VOCs as it can be adapted to different organic emissions under mild conditions. This review first introduces the hazards of VOCs, their treatment technologies, and summarizes the treatment mechanism issues. Next, the characteristics and catalytic performance of perovskite oxides as catalysts for VOC removal are expounded, with a special focus on lattice distortions and surface defects caused by metal doping and surface modifications, and on the treatment of different VOCs. The challenges and the prospects regarding the design of perovskite oxides catalysts for the catalytic combustion of VOCs are also discussed. This review provides a reference base for improving the performance of perovskite catalysts to treat VOCs.

Keywords perovskite oxides volatile organic compounds catalytic combustion reaction mechanism

Corresponding Author(s): Junjiang Zhu,Xinying Liu

About author:

Peng Lei and Charity Ngina Mwangi contributed equally to this work.

Just Accepted Date: 15 May 2023 Online First Date: 03 July 2023 Issue Date: 25 October 2023

Cite this article:

Shan Wang,Ping Xiao,Jie Yang, et al. Catalytic combustion of volatile organic compounds using perovskite oxides catalysts—a review[J]. Front. Chem. Sci. Eng., 2023, 17(11): 1649-1676.

URL:

https://academic.hep.com.cn/fcse/EN/10.1007/s11705-023-2324-x
https://academic.hep.com.cn/fcse/EN/Y2023/V17/I11/1649

Tab.1 Common types of VOCs

Fig.1 Relationship between VOCs, O₃ and PM_2.5.

Tab.2 Conditions used in common VOCs control technologies [40]

Tab.3 Comparison of different combustion processes [50]

Fig.3 Crystal structure of (a) the ideal ABO₃-type perovskite oxides, (b) Ruddlesden–Popper (RP) series of layered perovskite oxides (A_{n + 1}B_nO_{3n + 1}), (c) A-site ordered double perovskite oxides (AA’B₂O₆) and (d) B-site ordered double perovskite oxides (A₂BB’O₆). Reprinted with permission from Ref. [73], copyright 2020, Royal Society of Chemistry.

Tab.4 Survey of literature data on the catalytic oxidation of toluene at low temperature

Fig.4 (a) Migration and transformation mechanism of surface reactive oxygen in SmMnO₃. Used with permission from [90], copyright 2019 American Chemical Society; (b) Preparation route of γ-MnO₂/SmMnO₃ catalyst. Reprinted with permission from Ref. [99], copyright 2019, Elsevier.

Fig.5 Catalytic mechanism and main reactive oxygen species of La_n+1Ni_nO_3n+1 layered perovskites for catalytic oxidation of methane and toluene. Reprinted with permission from Ref. [86], copyright 2016, American Chemical Society.

Fig.6 (a) Vacancy formation energies, (b) O atom desorption energy, (c) propane adsorption energies, and (d) propane dissociation on La and the Co-exposed surface. Reprinted with permission from Ref. [130], copyright 2022, Elsevier.

Tab.5 Perovskite oxides catalysts for catalytic combustion of VOCs

Fig.9 (a) The catalytic activity of toluene oxidation over Ag substituted LaCoO₃ catalysts (250, 450 and 700 represent the calculation temperatures, in °C). Reprinted with permission from Ref. [168], copyright 2019, Elsevier. (b) Schematic diagram of La_0.9CoO_3–δ catalytic oxidation of toluene. Reprinted with permission from Ref. [169], copyright 2023, Elsevier.

Fig.10 (a) Schematic illustration of SMO synthesis; (b) toluene conversion versus reaction temperature over SMO-N, SMO-G and SMO-B; (c) Arrhenius plots of the three samples used for toluene oxidation; (d) effect of weight hourly space velocity on toluene oxidation over SMO-N; (e) CO₂ yield from toluene, benzene and o-xylene oxidation versus reaction temperature over SMO-N. Reprinted with permission from Ref. [170], copyright 2018, American Chemical Society.

Fig.11 (a) Product distribution after 6 h on stream for several Rh/perovskite catalysts; (b) product distribution of the catalytic test and ethanol conversion during 24 h of reaction for the Rh/LaAlO₃ 0.3% catalyst (right). Reprinted with permission from Ref. [175], copyright 2021, Elsevier.

Fig.12 (a) Configuration of intermediates and reaction cycle of HCHO oxidation on an Ag-LMO catalyst. Reprinted with permission from Ref. [178], copyright 2022, Elsevier. (b) Reaction mechanism of HCHO oxidation on La_1–x(Sr, Na, K)_xMnO₃. Reprinted with permission from Ref. [179], copyright 2021, Elsevier.

Fig.13 (a) Possible major reaction pathways in the plasma removal of EA. Reprinted with permission from Ref. [190], copyright 2017, Elsevier. (b) Mechanism proposed for the catalytic oxidation of EA. Reprinted with permission from Ref. [149], copyright 2022, Elsevier.

Fig.14 Reaction mechanism pathways proposed for 1,2-DCP catalytic oxidation over LaMnO₃ perovskite under oxygenated conditions and inert conditions. Reprinted with permission from Ref. [196], copyright 2021, Elsevier.

Fig.15 (a) Reaction energy profile and structures of intermediates; (b) The reaction cycle for CH₂Cl₂ elimination on LaMnO₃(010) catalyst. Reprinted with permission from Ref. [200], copyright 2021, Elsevier.

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