Activated carbons and amine-modified materials for carbon dioxide capture –– a review

doi:10.1007/s11783-013-0510-7

Front Envir Sci Eng

0, Vol.

Issue () : 326-340 https://doi.org/10.1007/s11783-013-0510-7

REVIEW ARTICLE

Activated carbons and amine-modified materials for carbon dioxide capture –– a review

Zhenhe CHEN¹, Shubo DENG^1,2(

), Haoran WEI¹, Bin WANG¹, Jun HUANG¹, Gang YU^1,2

1. State Key Joint Laboratory of Environment Simulation and Pollution Control, School of Environment, POPs Research Center, Tsinghua University, Beijing 100084, China; 2. Tsinghua University – Veolia Environment Joint Research Center for Advanced Technology, Tsinghua University, Beijing 100084, China

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Abstract

Rapidly increasing concentration of CO₂ in the atmosphere has drawn more and more attention in recent years, and adsorption has been considered as an effective technology for CO₂ capture from the anthropogenic sources. In this paper, the attractive adsorbents including activated carbons and amine-modified materials were mainly reviewed and discussed with particular attention on progress in the adsorbent preparation and CO₂ adsorption capacity. Carbon materials can be prepared from different precursors including fossil fuels, biomass and resins using the carbonization-activation or only activation process, and activated carbons prepared by KOH activation with high CO₂ adsorbed amount were reviewed in the preparation, adsorption capacity as well as the relationship between the pore characteristics and CO₂ adsorption. For the amine-modified materials, the physical impregnation and chemical graft of polyethylenimine (PEI) on the different porous materials were introduced in terms of preparation method and adsorption performance as well as their advantages and disadvantages for CO₂ adsorption. In the last section, the issues and prospect of solid adsorbents for CO₂ adsorption were summarized, and it is expected that this review will be helpful for the fundamental studies and industrial applications of activated carbons and amine-modified adsorbents for CO₂ capture.

Keywords adsorption capacity CO₂ capture activated carbon amine-impregnated adsorbents

Corresponding Author(s): DENG Shubo,Email:dengshubo@tsinghua.edu.cn

Issue Date: 01 June 2013

Cite this article:

Zhenhe CHEN,Shubo DENG,Haoran WEI, et al. Activated carbons and amine-modified materials for carbon dioxide capture –– a review[J]. Front Envir Sci Eng, 0, (): 326-340.

URL:

https://academic.hep.com.cn/fese/EN/10.1007/s11783-013-0510-7
https://academic.hep.com.cn/fese/EN/Y0/V/I/326

Tab.1 Components and characteristics of flue gas and air

Tab.2 Comparison of different adsorbents for CO capture

Tab.3 CO uptake on different carbon materials prepared by different methods

Tab.4 PEI-impregnated adsorbents for CO capture

Fig.1 Effects of PEI molecular weights and the pore characteristics of the porous materials on CO adsorption on the PEI-impregnated adsorbents

Tab.5 CO uptake on different amine-grafted adsorbents

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