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Multiphase redistribution differences of polycyclic aromatic hydrocarbons (PAHs) between two successive sediment suspensions |
Rufeng LI,Chenghong FENG( ),Dongxin WANG,Baohua LI,Zhenyao SHEN |
The Key Laboratory of Water and Sediment Sciences (Ministry of Education), School of Environment, Beijing Normal University, Beijing 100875, China |
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Abstract Successive sediment suspensions often happen in estuary, yet little research has probed into the difference in the release behaviors of organic compounds among different suspensions. This study took polycyclic aromatic hydrocarbons (PAHs) as typical organic contaminants and investigated the release behaviors between two successive suspensions with a particle entrainment simulator (PES). Results showed that successive sediment suspensions lowered the concentration of dissolved PAHs in the overlying water via facilitating the re-adsorption of dissolved PAHs onto the suspended particles. Fast-release and slow-release periods of PAHs were successively observed in the both suspensions. The concentration changes of dissolved PAHs in the second suspension were generally similar with but hysteretic to those in the first suspension. More vigorous desorption and re-absorption of PAHs were induced in the second suspension. Successive sediment suspensions obviously decreased the concentrations of mineral composition and organic matters in the overlying water, which significantly affects multiphase distribution of PAHs.
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Keywords
sediment suspension
PAHs
multiphase distribution
distribution coefficients
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Corresponding Author(s):
Chenghong FENG
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Online First Date: 17 September 2015
Issue Date: 01 February 2016
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