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Frontiers of Environmental Science & Engineering

ISSN 2095-2201

ISSN 2095-221X(Online)

CN 10-1013/X

Postal Subscription Code 80-973

2018 Impact Factor: 3.883

Front. Environ. Sci. Eng.    2022, Vol. 16 Issue (3) : 29    https://doi.org/10.1007/s11783-021-1463-x
RESEARCH ARTICLE
Four kinds of capping materials for controlling phosphorus and nitrogen release from contaminated sediment using a static simulation experiment
Zhenming Zhou(), Canyang Lin, Shuwen Li, Shupo Liu, Fei Li, Baoling Yuan
College of Civil Engineering, Huaqiao University, Xiamen 361021, China
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Abstract

• Lanthanum modified bentonite (LMB) can effectively absorb phosphorus (P).

• Water treatment plant sludge (WTPS) capping is effective for controlling P release.

•Aluminum-based P-inactivation agent (Al-PIA) is an efficient P control material.

•The P adsorbed by WTPS and Al-PIA is mainly in the form of NAIP.

We determined the effects of quartz sand (QS), water treatment plant sludge (WTPS), aluminum-based P-inactivation agent (Al-PIA), and lanthanum-modified bentonite (LMB) thin-layer capping on controlling phosphorus and nitrogen release from the sediment, using a static simulation experiment. The sediment in the experiment was sampled from Yundang Lagoon (Xiamen, Fujian Province, China), which is a eutrophic waterbody. The total phosphorus (TP), ammonium nitrogen (NH4+-N), and total organic carbon (TOC) levels in the overlying water were measured at regular intervals, and the changes of different P forms in WTPS, Al-PIA, and sediment of each system were analyzed before and after the test. The average TP reduction rates of LMB, Al-PIA, WTPS, and QS were 94.82, 92.14, 86.88, and 10.68%, respectively, when the release strength of sediment TP was 2.26–9.19 mg/(m2·d) and the capping strength of the materials was 2 kg/m2. Thin-layer capping of LMB, WTPS, and Al-PIA could effectively control P release from the sediment (P<0.05). However, thin-layer capping of LMB, Al-PIA, and QS did not significantly reduce the release of ammonium N and organic matter (P > 0.05). Based on our results, LMB, Al-PIA, and WTPS thin-layer capping promoted the migration and transformation of easily released P in sediment. The P adsorbed by WTPS and Al-PIA mainly occurred in the form of NAIP.

Keywords Sediment      Eutrophication      Thin-layer capping      Phosphorus      Nitrogen      Aluminum-based P-inactivation agent     
Corresponding Author(s): Zhenming Zhou   
Issue Date: 13 July 2021
 Cite this article:   
Zhenming Zhou,Canyang Lin,Shuwen Li, et al. Four kinds of capping materials for controlling phosphorus and nitrogen release from contaminated sediment using a static simulation experiment[J]. Front. Environ. Sci. Eng., 2022, 16(3): 29.
 URL:  
https://academic.hep.com.cn/fese/EN/10.1007/s11783-021-1463-x
https://academic.hep.com.cn/fese/EN/Y2022/V16/I3/29
Fig.1  Schematic of the experimental glass bottle. ① Glass bottle; ② Overlying water; ③ Capping materials; ④ Sediment.
Fig.2  The protocols of SMT extraction.
Fig.3  Changes of TP concentrations of overlying water in the five systems.
Fig.4  Changes of NH4+-N concentrations of overlying water in the five systems.
Sample Ammonium nitrogen content (mg/kg) Organic matter content (mg/kg)
WTPS Before reaction 156.86±1.08 163.69±0.24
After reaction 46.16±0.22 91.64±2.51
Al-PIA Before reaction 57.42±0.86 38.32±0.08
After reaction 38.90±0.65 35.94±0.47
Tab.1  Changes of various forms of ammonium nitrogen and organic matter content in WTPS and Al-PIA before and after tests
Fig.5  Changes of TOC concentrations of overlying water in the five systems.
Fig.6  Changes of various forms of phosphorus content in the WTPS and Al-PIA.
Fig.7  Changes of phosphorus content of sediment in different systems.
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