A direct method to calculate second-order two-dimensional terahertz spectroscopy in frequency-domain based on classical theory

doi:10.1007/s12200-018-0863-4

Front. Optoelectron.

2018, Vol. 11

Issue (4) : 413-418 https://doi.org/10.1007/s12200-018-0863-4

RESEARCH ARTICLE

A direct method to calculate second-order two-dimensional terahertz spectroscopy in frequency-domain based on classical theory

Feidi XIANG, Kejia WANG(

), Zhengang YANG, Jinsong LIU, Shenglie WANG

Wuhan National Laboratory for Optoelectronics, School of Optical and Electronic information, Huazhong University of Science and Technology, Wuhan 430074, China

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Abstract

Previous theoretical researches on the two-dimensional terahertz spectroscopy (2DTS), which are conducted via inefficiently time-consuming numerical simulation, deal with only single-mode system. To overcome the limitations, we derive a classical-theory-based analytical solution which is applicable to multi-modes system. Three typical weak sources of nonlinearities are introduced. The findings suggest that the analytical results correspond well with those obtained by the traditional numerical simulation. Thus the study provides a more efficient and practical method to directly calculate 2DTS, and, in a broader sense, sheds new light on the theory of 2DTS.

Keywords two-dimensional spectroscopy terahertz classical method

Corresponding Author(s): Kejia WANG

Just Accepted Date: 20 November 2018 Online First Date: 14 December 2018 Issue Date: 21 December 2018

Cite this article:

Feidi XIANG,Kejia WANG,Zhengang YANG, et al. A direct method to calculate second-order two-dimensional terahertz spectroscopy in frequency-domain based on classical theory[J]. Front. Optoelectron., 2018, 11(4): 413-418.

URL:

https://academic.hep.com.cn/foe/EN/10.1007/s12200-018-0863-4
https://academic.hep.com.cn/foe/EN/Y2018/V11/I4/413

Fig.1 Timing schematic diagram of 2DTS

Fig.2 THz pulse used in calculation shown in time- (a) and frequency- (b) domain

Fig.3 Normalized 2D diagrams corresponding to (a) AH, (b) NC, and (c) ND obtained by analytical calculation, and those corresponding to (d) AH, (e) NC, and (f) ND obtained by numerical simulation. Only the first quartile is presented to display more details

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