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Efficient removal and upcycling of pollutants in wastewater: a strategy for reconciling environmental pollution and resource depletion crisis |
Lei Bi1,2, Qiong Wang1,2, Jingzhang Liu1,2, Fuxiang Cui1,2, Maoyong Song1,2( ) |
1. Key Laboratory of Environmental Nanotechnology and Health Effects, Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences, Beijing 100085, China 2. University of Chinese Academy of Sciences, Beijing 100049, China |
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Abstract Due to the relentless exploitation of non-renewable resources, humanity is faced with a resource depletion crisis in the coming decades and serious environmental issues. Achieving efficient removal and upcycling of pollutants (ERUP) may become a potential strategy to address these issues. Wastewater, characterized by its large production volume and fluidity, can easily cause widespread environmental pollution through natural water networks. Due to solubility constraints, pollutants in wastewater typically exhibit low concentrations and complex compositions, thereby impeding effective recovery. Therefore, achieving ERUP in wastewater is both highly significant and extremely challenging. Unlike conventional wastewater treatment strategies that are focused on removing pollutants, ERUP strategies can not only realize the efficient removal of pollutants from water but also convert pollutants into valuable and functional products. Herein, we enumerated the latest research progress on ERUP in wastewater and highlighted studies that demonstrate the simultaneous achievement of pollutant removal and the direct conversion of these contaminants into high-efficiency catalysts, hydrogen energy, electrical energy, and other high-value chemicals. Finally, we identified the problems and challenges in the development of ERUP in wastewater and outlined potential research directions for future studies.
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Keywords
environmental pollution
resource depletion
upcycling
wastewater
pollutants
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Corresponding Author(s):
Maoyong Song
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About author: #These authors contributed equally to this work. |
Just Accepted Date: 13 June 2024
Issue Date: 09 August 2024
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1 |
R M DuChanois , N J Cooper , B Lee , S K Patel , L Mazurowski , T E Graedel , M Elimelech . Prospects of metal recovery from wastewater and brine. Nature Water, 2023, 1(1): 37–46
https://doi.org/10.1038/s44221-022-00006-z
|
2 |
L Tozer. Water pollution ‘timebomb’ threatens global health. Nature, July 18, 2023. https://doi.org/10.1038/d41586–023-01586–023
|
3 |
R D Cusick , Y Kim , B E Logan . Energy capture from thermolytic solutions in microbial reverse-electrodialysis cells. Science, 2012, 335(6075): 1474–1477
https://doi.org/10.1126/science.1219330
|
4 |
L Bi , Y P Chen , C Wang , J Su , G Pan . Microalgae-derived cellulose/inorganic nanocomposite rattle-type microspheres as an advanced sensor for pollutant detection. Chemical Engineering Journal, 2020, 395: 125073
https://doi.org/10.1016/j.cej.2020.125073
|
5 |
L Bi , X Luan , F L Geng , X Xu , Y P Chen , F Zhang . Microwave-assisted synthesis of hollow microspheres with multicomponent nanocores for heavy-metal removal and magnetic sensing. ACS Applied Materials & Interfaces, 2020, 12(41): 46779–46787
https://doi.org/10.1021/acsami.0c14298
|
6 |
L Bi , J Z Liu , M Du , B Huang , M Y Song , G B Jiang . In-situ upcycling of cadmium from wastewater into core-shell ZnS@Zn0.58Cd0.42S heterojunction photocatalyst for environmental purification and H2 evolution. Chemical Engineering Journal, 2023, 454: 140258
https://doi.org/10.1016/j.cej.2022.140258
|
7 |
S Wang , D Zhang , W Wang , J Zhong , K Feng , Z Wu , B Du , J He , Z Li , L He . et al.. Grave-to-cradle upcycling of Ni from electroplating wastewater to photothermal CO2 catalysis. Nature Communications, 2022, 13(1): 5305
https://doi.org/10.1038/s41467-022-33029-x
|
8 |
B Wang , X Xiao , J Li , M Zhang , M Jiao , Z Zheng , T Li , Q Zhang , X Zhang , G Zhou . Sulfion oxidation assisting self-powered hydrogen production system based on efficient catalysts from spent lithium-ion batteries. Proceedings of the National Academy of Sciences of the United States of America, 2023, 120(52): e2317174120
https://doi.org/10.1073/pnas.2317174120
|
9 |
K Zheng , Y Wang , L Xiang , C Huang , H Zhang , J Li . A dual-cycle regeneration to recover high-value and high-purity FePO4 from real wastewater for Li-battery application. Water Research, 2023, 242: 120300
https://doi.org/10.1016/j.watres.2023.120300
|
10 |
W Wang , J Chen , E C M Tse . Synergy between Cu and Co in a layered double hydroxide enables close to 100% nitrate-to-ammonia selectivity. Journal of the American Chemical Society, 2023, 145(49): 26678–26687
https://doi.org/10.1021/jacs.3c08084
|
11 |
S An , Z H Zhao , J Bu , J He , W Ma , J Lin , R Bai , L Shang , J Zhang . Multi-functional formaldehyde-nitrate batteries for wastewater refining, electricity generation, and production of ammonia and formate. Angewandte Chemie International Edition, 2024, 63(11): e202318989
https://doi.org/10.1002/anie.202318989
|
12 |
X Z Fu , Y R Yang , T Liu , Z Y Guo , C X Li , H Y Li , K P Cui , W W Li . Biological upcycling of nickel and sulfate as electrocatalyst from electroplating wastewater. Water Research, 2024, 250: 121063
https://doi.org/10.1016/j.watres.2023.121063
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