Latest advances in ionic liquids promoted synthesis and application of advanced biomass materials

doi:10.1007/s11705-023-2316-x

Front. Chem. Sci. Eng.

2023, Vol. 17

Issue (7) : 798-816 https://doi.org/10.1007/s11705-023-2316-x

REVIEW ARTICLE

Latest advances in ionic liquids promoted synthesis and application of advanced biomass materials

Ting He¹, Jipeng Yan¹, Wenzhe Xiao¹, Jian Sun^1,²(

)

¹. Key Laboratory of Molecular Medicine and Biotherapy in the Ministry of Industry and Information Technology, School of Life Science, Beijing Institute of Technology, Beijing 100081, China
². Beijing Engineering Research Center of Cellulose and Its Derivatives, Advanced Research Institute of Multidisciplinary Science, Beijing Institute of Technology, Beijing 100081, China

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Abstract

The utilization of sustainable resources provides a path to relieving the problem of dependence on fossil resources. In this context, biomass materials have become a feasible substitute for petroleum-based materials. The development of biomass materials is booming and advanced biomass materials with various functional properties are used in many fields including medicine, electrochemistry, and environmental science. In recent years, ionic liquids have been widely used in biomass pretreatments and processing owing to their “green” characteristics and adjustable physicochemical properties. Thus, the effects of ionic liquids in biomass materials generation require further study. This review summarizes the multiple roles of ionic liquids in promoting the synthesis and application of advanced biomass materials as solvents, structural components, and modifiers. Finally, a prospective approach is proposed for producing additional higher-quality possibilities between ionic liquids and advanced biomass materials.

Keywords biomass materials functional materials ionic liquids synthesis structure-property relationship

Corresponding Author(s): Jian Sun

About author:

^* These authors contributed equally to this work.

Just Accepted Date: 17 March 2023 Online First Date: 12 June 2023 Issue Date: 05 July 2023

Cite this article:

Ting He,Jipeng Yan,Wenzhe Xiao, et al. Latest advances in ionic liquids promoted synthesis and application of advanced biomass materials[J]. Front. Chem. Sci. Eng., 2023, 17(7): 798-816.

URL:

https://academic.hep.com.cn/fcse/EN/10.1007/s11705-023-2316-x
https://academic.hep.com.cn/fcse/EN/Y2023/V17/I7/798

Fig.1 (a) This statistical graph is based on published data retrieved on the Web of Science by the keyword “biomass materials”, Nov. 19th, 2022; (b) this heat map is based on data from Web of Science, Nov. 19th, 2022, and analyzed by a VOS viewer.

Fig.2 Schematic diagram of ILs promoting the synthesis and application of advanced biomass materials.

Fig.3 Typical routes for the pretreatment of lignocellulosic biomass with ILs. Reprinted from Ref. [36].

Fig.4 Scanning electron microscopy (SEM) images of beads prepared from (a) commercially available chitin and (b) IL-extracted chitin (The beads size fraction used for imaging was > 250 μm). Reprinted with permission from Ref. [51], copyright 2017, American Chemical Society.

Fig.5 (a) Absorption spectra of RCCDs (Inset: optical images under daylight (left) and 365-nm UV light (right)); (b) excitation-dependent emission photoluminescence (PL) spectra of RCCDs at different wavelengths, increasing from 340 to 440 nm with 20 nm increments (Inset: normalized PL emission spectra). Reprinted with permission from Ref. [59], copyright 2018, American Chemical Society.

Fig.9 Three different conducting mechanisms for composite CNT temperature sensors. (i–iii) Three different electron/ions transport modes in CNT and [Emim][NTf₂] composite sensing materials: (i) the transport of charges via the body-body contacts among CNTs; (ii) the transport via the end-to-end contacts of CNTs; (iii) the transport via ILs. Reprinted with permission from Ref. [90], copyright 2019, Wiley.

Fig.10 (a) SEM images of E. coli, S. aureus, and C. albicans before treatment (control) and after treatment using the ionogel; (b) schematic diagram of the antibacterial mechanism of ionogel. Reprinted with permission from Ref. [94], copyright 2021, Royal Society of Chemistry.

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